ترغب بنشر مسار تعليمي؟ اضغط هنا

Interplay between magnetic and lattice excitations in BiFeO$_3$

239   0   0.0 ( 0 )
 نشر من قبل Maximilien Cazayous
 تاريخ النشر 2008
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman spectra has been previously assigned to two phonon overtone. We show here that its unusual frequency shift with the excitation energy and its asymmetric temperature dependent Fano lineshape reveal a strong coupling to magnetic excitations. In the same energy range, we have also identified the two-magnon excitation with a temperature dependence very similar to $alpha$-Fe$_2$O$_3$ hematite.

قيم البحث

اقرأ أيضاً

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the magneto-act ive modes, i.e. antiferromagnetic resonances (AFMR). Two AFMR resonances were found to coincide with electromagnons. This indicates that both excitations belong to the same mode and the electromagnons can be excited by magnetic ac-field as well. In external magnetic fields and at low temperatures distinct fine structure of the electromagnons appears. In spite of the 90^o rotation of the magnetic structure, the electromagnons are observable for electric ac-fields parallel to the a-axis only. Contrary to simple expectations, the response along the c-axis remains purely magnetic in nature.
We have studied the magnetic field dependence of far-infrared active magnetic modes in a single ferroelectric domain BFO/ crystal at low temperature. The modes soften close to the critical field of 18.8,T along the [001] (pseudocubic) axis, where the cycloidal structure changes to the homogeneous canted antiferromagnetic state and a new strong mode with linear field dependence appears that persists at least up to 31,T. A microscopic model that includes two DM/ interactions and easy-axis anisotropy describes closely both the zero-field spectroscopic modes as well as their splitting and evolution in a magnetic field. The good agreement of theory with experiment suggests that the proposed model provides the foundation for future technological applications of this multiferroic material.
219 - J. Bobroff , S. Hebert , G. Lang 2007
We present a comparative study of CoO2 layers in the Bi-misfit and NaxCoO2 cobaltates. Co NMR measures the intrinsic susceptibility of the Co layers and is not affected by spurious contributions. At low dopings where room-temperature thermopower (TEP ) is large, Curie-Weiss susceptibilities are observed in both materials. But NMR and muSR experiments find neither charge nor spin order down to low temperatures in Bi-misfit, in contrast to the case of NaxCoO2. This demonstrates that metallicity, charge and magnetic orders are specific of the Na layers in NaxCoO2 whereas strong correlations are generic of the cobaltates physics and could explain the large TEP.
129 - B. Xu , P. Marsik , S. Sarkar 2021
We report an infrared spectroscopy study of the axion topological insulator candidate EuIn$_2$As$_2$ for which the Eu moments exhibit an A-type antiferromagnetic (AFM) order below $T_N simeq 18 mathrm{K}$. The low energy response is composed of a wea k Drude peak at the origin, a pronounced infrared-active phonon mode at 185 cm$^{-1}$ and a free carrier plasma edge around 600 cm$^{-1}$. The interband transitions start above 800 cm$^{-1}$ and give rise to a series of weak absorption bands at 5,000 and 12,000 cm$^{-1}$ and strong ones at 20,000, 27,500 and 32,000 cm$^{-1}$. The AFM transition gives rise to pronounced anomalies of the charge response in terms of a cusp-like maximum of the free carrier scattering rate around $T_N$ and large magnetic splittings of the interband transitions at 5,000 and 12,000 cm$^{-1}$. The phonon mode at 185 cm$^{-1}$ has also an anomalous temperature dependence around $T_N$ which suggests that it couples to the fluctuations of the Eu spins. The combined data provide evidence for a strong interaction amongst the charge, spin and lattice degrees of freedom.
The spin-driven component of electric polarization in a single crystal of multiferroic BiFeO$_{3}$ was experimentally investigated in pulsed high magnetic fields up to 41 T. Sequential measurements of electric polarization for various magnetic field directions provide clear evidence of electric polarization normal to the hexagonal $c$ axis (${bf P}_{rm t}$) in not only the cycloidal phase, but also the field-induced canted antiferromagnetic phase. The direction of ${bf P}_{rm t}$ is directly coupled with the ferromagnetic moment in the canted antiferromagnetic phase, and thus controlled by changing the direction of the applied magnetic field. This magnetoelectric coupling is reasonably reproduced by the metal-ligand hybridization model.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا