ترغب بنشر مسار تعليمي؟ اضغط هنا

Nature of the field-induced magnetic incommensurability in multiferroic Ni$_3$TeO$_6$

61   0   0.0 ( 0 )
 نشر من قبل Jakob Lass
 تاريخ النشر 2019
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Using single crystal neutron scattering we show that the magnetic structure Ni$_3$TeO$_6$ at fields above 8.6 T along the $c$ axis changes from a commensurate collinear antiferromagnetic structure with spins along c and ordering vector $Q_C$= (0 0 1.5), to a conical spiral with propagation vector $Q_{IC}$= (0 0 1.5$pmdelta$),$deltasim$0.18, having a significant spin component in the ($a$,$b$) plane. We determine the phase diagram of this material in magnetic fields up to 10.5 T along $c$ and show the phase transition between the low field and conical spiral phases is of first order by observing a discontinuous jump of the ordering vector. $Q_{IC}$ is found to drift both as function of magnetic field and temperature. Preliminary inelastic neutron scattering reveals that the spin wave gap in zero field has minima exactly at $Q_{IC}$ and a gap of about 1.1 meV consisting with a cross-over around 8.6 T. Our findings excludes the possibility of the inverse Dzyaloshinskii-Moriya interaction as a cause for the giant magneto-electric coupling earlier observed in this material and advocates for the symmetric exchangestriction as the origin of this effect.



قيم البحث

اقرأ أيضاً

211 - Song Bao , Zhengwei Cai , Wenda Si 2020
We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific heat and th ermal conductivity results show that the thermal transport is dominated by phonons, the deviation of the thermal conductivity from a pure phononic model indicates that there is a strong coupling between magnons and phonons. In the INS measurements, we find a mode in the excitation spectra at 4.5 K, which exhibits a slight downward dispersion around the Brillouin zone center. This mode disappears above the N{e}el temperature, and thus cannot be a phonon. Furthermore, the dispersion is distinct from that of a magnon. Instead, it can be explained by the magnon-polaron mode, which is new collective excitations resulting from the hybridization between magnons and phonons. We consider the suppression of the thermal conductivity and emergence of the magnon-polaron mode to be evidence for magnon-phonon coupling in Cu$_3$TeO$_6$.
Ab initio calculations have been performed to unravel the origin of the recently found superlattice peaks in the trilayer nickelate La$_4$Ni$_3$O$_8$. These peaks arise from static charge ordering of Ni$^{2+}$/ Ni$^{1+}$ stripes oriented at 45$^{circ }$ to the Ni-O bonds. An insulating state originates from a combination of structural distortions and magnetic order, with the gap being formed solely within the d$_{x^2-y^2}$ manifold of states. When doped, electrons or holes would go into these states, in a similar fashion to what occurs in the cuprates. Analogous calculations suggest that checkerboard charge order should occur in the bilayer nickelate La$_3$Ni$_2$O$_6$. These results reveal a close connection between La$_4$Ni$_3$O$_8$ and La$_3$Ni$_2$O$_6$ with La$_{2-x}$Sr$_x$NiO$_4$ for x=1/3 and x=1/2, respectively.
We report a magnetic x-ray scattering study of the field-induced multiferroic GdFe3(BO3)4. Resonant x-ray magnetic scattering at the Gd LII,III edges indicates that the Gd moments order at TN ~ 37 K. The magnetic structure is incommensurate below TN, with the incommensurability decreasing monotonically with decreasing temperature until a transition to a commensurate magnetic phase is observed at T ~ 10 K. Both the Gd and Fe moments undergo a spin reorientation transition at TSR ~ 9 K such that the moments are oriented along the crystallographic c axis at low temperatures. With magnetic field applied along the a axis, our measurements suggest that the field-induced polarization phase has a commensurate magnetic structure with Gd moments rotated ~45 degrees toward the basal plane, which is similar to the magnetic structure of the Gd subsystem observed in zero field between 9 and 10 K, and the Fe subsystem has a ferromagnetic component in the basal plane.
We present a $^{125}$Te nuclear magnetic resonance (NMR) study in the three-dimensional spin web lattice Cu$_3$TeO$_6$, which harbors topological magnons. The $^{125}$Te NMR spectra and the Knight shift $mathcal{K}$ as a function of temperature show a drastic change at $T_text{S}sim 40$ K much lower than the Neel ordering temperature $T_text{N}sim 61$ K, providing evidence for the first-order structural phase transition within the magnetically ordered state. Most remarkably, the temperature dependence of the spin-lattice relaxation rate $T_1^{-1}$ unravels spin-gap-like magnetic excitations, which sharply sets in at $T^*sim 75$ K, the temperature well above $T_text{N}$. The spin gap behavior may be understood by weakly dispersive optical magnon branches of high-energy spin excitations originating from the unique corner-sharing Cu hexagon spin-1/2 network with low coordination number.
Co$^{2+}$ ions in an octahedral crystal field, stabilise a j$_{eff}$ = 1/2 ground state with an orbital degree of freedom and have been recently put forward for realising Kitaev interactions, a prediction we have tested by investigating spin dynamics in two cobalt honeycomb lattice compounds, Na$_2$Co$_2$TeO$_6$ and Na$_3$Co$_2$SbO$_6$, using inelastic neutron scattering. We used linear spin wave theory to show that the magnetic spectra can be reproduced with a spin Hamiltonian including a dominant Kitaev nearest-neighbour interaction, weaker Heisenberg interactions up to the third neighbour and bond-dependent off-diagonal exchange interactions. Beyond the Kitaev interaction that alone would induce a quantum spin liquid state, the presence of these additional couplings is responsible for the zigzag-type long-range magnetic ordering observed at low temperature in both compounds. These results provide evidence for the realization of Kitaev-type coupling in cobalt-based materials, despite hosting a weaker spin-orbit coupling than their 4d and 5d counterparts.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا