ترغب بنشر مسار تعليمي؟ اضغط هنا

A Knotted Meta-molecule with 2-D Isotropic Optical Activity Rotating the Incident Polarization by 90{deg}

113   0   0.0 ( 0 )
 نشر من قبل Wending Mai
 تاريخ النشر 2019
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Optical activity is the ability of chiral materials to rotate linearly-polarized (LP) electromagnetic waves. Because of their intrinsic asymmetry, traditional chiral molecules usually lack isotropic performance, or at best only possess a weak form of chirality. Here we introduce a knotted chiral meta-molecule that exhibits optical activity corresponding to a 90{deg} polarization rotation of the incident waves. More importantly, arising from the continuous multi-fold rotational symmetry of the chiral torus knot structure, the observed polarization rotation behavior is found to be independent of how the incident wave is polarized. In other words, the proposed chiral knot structure possesses two-dimensional (2-D) isotropic optical activity as illustrated in Fig. 1, which has been experimentally validated in the microwave spectrum. The proposed chiral torus knot represents the most optically active meta-molecule reported to date that is intrinsically isotropic to the incident polarization.

قيم البحث

اقرأ أيضاً

117 - Vincent Jacques 2007
We report an optical technique that yields an enhancement of single-molecule photostability, by greatly suppressing photobleaching pathways which involve photoexcitation from the triplet state. This is accomplished by dynamically switching off the ex citation laser when a quantum-jump of the molecule to the triplet state is optically detected. This procedure leads to a lengthened single-molecule observation time and an increased total number of detected photons. The resulting improvement in photostability unambiguously confirms the importance of photoexcitation from the triplet state in photobleaching dynamics, and may allow the investigation of new phenomena at the single-molecule level.
82 - Yuqian Ye , Sailing He 2010
A bilayered chiral metamaterial (CMM) is proposed to realize a 90 degree polarization rotator, whose giant optical activity is due to the transverse magnetic dipole coupling among the metallic wire pairs of enantiomeric patterns. By transmission thro ugh this thin bilayered structure of less than lambda/30 thick, a linearly polarized wave is converted to its cross polarization with a resonant polarization conversion efficiency (PCE) of over 90%. Meanwhile, the axial ratio of the transmitted wave is better than 40 dB. It is demonstrated that the chirality in the propagation direction makes this efficient cross-polarization conversion possible. The transversely isotropic property of this polarization rotator is also experimentally verified. The optical activity of the present structure is about 2700 degree/lambda, which is the largest optical activity that can be found in literature.
Strong coupling with single molecules in plasmonic picocavities has emerged as a resource for room-temperature quantum control with nanoscale light. Tip-based nanoprobes can measure the local dynamics of individual molecular picocavities, but the ove rhead associated with sampling an inhomogeneous picocavity distribution can be challenging for scalability. We propose a macroscopic approach in which an ensemble of molecular picocavities acts as a nonlinear plasmonic metamaterial. Using a quantum optics perspective, we study theoretical performance limits for optical cross-phase modulation in the system, taking into account realistic distributions of picocavity volumes and molecular transition frequencies. The medium nonlinearity is mediated by local strong coupling with the lowest vibronic emission sideband of individual organic chomophores. The local vacua change the refractive index of the medium at the frequency of a weak probe field $omega_p$, set to drive the bare zero-phonon absorption band. Refractive index variations $Delta n/n$ of a few percent, relative to a molecule-free scenario, are feasible with dilute ensembles. The probe phase evolution can be switched off in the presence of a signal field at a higher frequency $omega_s$, for intensities as low as 10 kW/cm$^2$. The mechanism for optical switching involves a novel ($omega_p+omega_s$) two-photon absorption channel, assisted by local vacuum fields. Our work paves the way for future studies of plasmonic metamaterials that exploit strong light-molecule interactions, for applications in optical state preparation and control.
We report on a test of Lorentz invariance performed by comparing the resonance frequencies of one stationary optical resonator and one continuously rotating on a precision air bearing turntable. Special attention is paid to the control of rotation in duced systematic effects. Within the photon sector of the Standard Model Extension, we obtain improved limits on combinations of 8 parameters at a level of a few parts in $10^{-16}$. For the previously least well known parameter we find $tilde kappa_{e-}^{ZZ} =(-1.9 pm 5.2)times 10^{-15}$. Within the Robertson-Mansouri-Sexl test theory, our measurement restricts the isotropy violation parameter $beta -delta -frac 12$ to $(-2.1pm 1.9)times 10^{-10}$, corresponding to an eightfold improvement with respect to previous non-rotating measurements.
Our work is concerned with the case of the solar molecule CN which presents conspicuous profiles of scattering polarization. We start by calculating accurate PES for the singlet and triplet electronic ground states in order to characterize the collis ions between the CN molecule in its $X ; ^2Sigma$ state and the hydrogen in its ground state $^2S$. The PES are included in the Schroodinger equation to obtain the scattering matrix and the probabilities of collisions. Depolarizing collisional rate coefficients are computed in the framework of the infinite order sudden approximation for temperatures ranging from $T= 2000$ K to $T= 15000$ K. Interpretation of the results and comparison between singlet and triplet collisional rate coefficients are detailed. We show that, for typical photospheric hydrogen density ($n_{H} = 10^{15}-10^{16}$ cm$^{-3}$), the $X ; ^2Sigma$ state of CN is partially or completely depolarized by isotropic collisions.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا