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Band-resolved frequency modulation spectroscopy is a common method to measure weak signals of radiative ensembles. When the optical depth of the medium is large, the signal drops exponentially and the technique becomes ineffective. In this situation, we show that a signal can be recovered when a larger modulation index is applied. Noticeably, this signal can be dominated by the natural linewidth of the resonance, regardless of the presence of inhomogeneous line broadening. We implement this technique on a cesium vapor, and then explore its main spectroscopic features. This work opens the road towards measurement of cooperative emission effects in bulk atomic ensemble.
Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm. Detection
With the uncertainty of the optical clocks improving to the order of 10-18, the probe light used to detect the clock transition has demonstrated nonnegligible Stark shift, provoking to precisely evaluate this shift. Here, we demonstrate a frequency m
Optical frequency standards, lasers stabilized to atomic or molecular transitions, are widely used in length metrology and laser ranging, provide a backbone for optical communications and lie at the heart of next-generation optical atomic clocks. Her
We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an ultrastable 1.55 $m
A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum systems dipole response. We develop an analytic description of the comb spectr