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تسجيل مستخدم جديدDirect observation of magnetic domain evolution in the vicinity of Verwey transition in Fe3O4 thin films
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We report a direct observation of magnetic domain evolution near the Verwey transition (TV) in Fe3O4 films. We found the stripe domains in the Fe3O4/Mg2TiO4 film while the irregular domains in the Fe3O4/MgO film and the similar characters of magnetic domains in the vicinity of TV for both samples: the bigger domain size and the higher contrast of the phase signal below TV and the more disordered domain images at TV. Remarkably, the magnetic behaviors can be well understood and the domain-wall energy and the demagnetizing energy can be calculated from the magnetic domains near TV in the Fe3O4/Mg2TiO4 film. Our work presents a demonstration of the low temperature magnetic domains and gives a new perspective to understand the Verwey transition in Fe3O4 thin films.
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We have systematically studied the evolution of magnetic properties, especially the coercivity and the remanence ratio in the vicinity of the Verwey transition temperature (TV ), of high-quality epitaxial Fe3O4 thin films grown on MgO (001), MgAl2O4
(MAO) (001), and SrTiO3 (STO) (001) substrates. We observed rapid change of magnetization, coercivity, and remanence ratio at TV , which are consistent with the behaviors of resistivity versus temperature [r{ho}(T )] curves for the different thin films. In particular, we found quite different magnetic behaviors for the thin films onMgOfrom those onMAOand STO, inwhich the domain size and the strain state play very important roles. The coercivity is mainly determined by the domain size but the demagnetization process is mainly dependent on the strain state. Furthermore, we observed a reversal of remanence ratio at TV with thickness for the thin films grown on MgO: from a rapid enhancement for 40-nm- to a sharp drop for 200-nm-thick film, and the critical thickness is about 80 nm. Finally, we found an obvious hysteretic loop of coercivity (or remanence ratio) with temperature around TV , corresponding to the hysteretic loop of the r{ho}(T ) curve, in Fe3O4 thin film grown on MgO.
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