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تسجيل مستخدم جديدOptimally Chiral Electromagnetic Fields: Helicity Density and Interaction of Structured Light with Nanoscale Matter
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We propose the concept of helicity maximization applicable to structured light and obtain a universal rela-tion for the maximum of helicity density at a given field energy density. We further demonstrate that us-ing structured light with maximized helicity density eliminates the need of the specific knowledge of en-ergy and helicity densities in determining the chirality of a nanoparticle. The helicity maximization con-cept generalizes the use of the dissymmetry factor in chirality detection to any chiral structure light il-luminating nanoparticles.
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Structured light enables the characterization of chirality of optically small nanoparticles by taking advantage of the helicity maximization concept recently introduced in[1]. By referring to fields with nonzero helicity density as chiral fields, we
first investigate the properties of two chiral optical beams in obtaining helicity density localization and maximization requirements. The investigated beams include circularly polarized Gaussian beams and also an optical beam properly composed by a combination of a radially and an azi-muthally polarized beam. To acquire further enhancement and localization of helicity density beyond the diffraction limit, we also study chiral fields at the vicinity of a spherical dielectric nanoantenna and demon-strate that the helicity density around such a nanoantenna is a superposition of helicity density of the illu-minating field, scattered field, and an interference helicity term. Moreover, we illustrate when the nanoan-tenna is illuminated by a proper combination of azimuthal and radially polarized beams, the scattered nearfields satisfy the helicity maximization conditions beyond the diffraction limit. The application of the concept of helicity maximization to nanoantennas and generating optimally chiral nearfield result in helici-ty enhancement which is of great advantage in areas like detection of nanoscale chiral samples, microsco-py, and optical manipulation of chiral nanoparticles.
Research on spatially-structured light has seen an explosion in activity over the past decades, powered by technological advances for generating such light, and driven by questions of fundamental science as well as engineering applications. In this r
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