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Optical pulses are routinely used to drive dynamical changes in the properties of solids. In quantum materials, many new phenomena have been discovered, including ultrafast transitions between electronic phases, switching of ferroic orders and nonequilibrium emergent behaviors such as photo-induced superconductivity. Understanding the underlying non-equilibrium physics requires detailed measurements of multiple microscopic degrees of freedom at ultrafast time resolution. Femtosecond x-rays are key to this endeavor, as they can access the dynamics of structural, electronic and magnetic degrees of freedom. Here, we cover a series of representative experimental studies in which ultrashort x-ray pulses from free electron lasers have been used, opening up new horizons for materials research.
We have developed a polarized hard X-ray photoemission (HAXPES) system to study the ground-state symmetry of strongly correlated materials. The linear polarization of the incoming X-ray beam is switched by the transmission-type phase retarder compose
Thermal transport is less appreciated in probing quantum materials in comparison to electrical transport. This article aims to show the pivotal role that thermal transport may play in understanding quantum materials: the longitudinal thermal transpor
Investigations of magnetically ordered phases on the femtosecond timescale have provided significant insights into the influence of charge and lattice degrees of freedom on the magnetic sub-system. However, short-range magnetic correlations occurring
Femtosecond (fs)-resolved simultaneous measurements of charge and spin dynamics reveal the coexistence of two different quasi-particle excitations in colossal magneto-resistive (CMR) manganites, with {em fs} and {em ps} relaxation times respectively.
We show that the macroscopic magnetic and electronic properties of strongly correlated electron systems can be manipulated by coupling them to a cavity mode. As a paradigmatic example we consider the Fermi-Hubbard model and find that the electron-cav