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Using density functional theory calculations, we have found an enhanced magneto-optical Kerr effect in Fe/insulator interfaces. The results of our study indicate that interfacial Fe atoms in the Fe films have a low-dimensional nature, which causes the following two effects: (i) The diagonal component $sigma_{xx}$ of the optical conductivity decreases dramatically because the hopping integral for electrons between Fe atoms is suppressed by the low dimensionality. (ii) The off-diagonal component $sigma_{xy}$ of the optical conductivity does not change at low photon energies, but it is enhanced at photon energies around 2 eV, where we obtain enhanced orbital magnetic moments and spin-orbit correlations for the interfacial Fe atoms. A large Kerr angle develops in proportion to the ratio $sigma_{xy}/sigma_{xx}$. Our findings indicate an efficient way to enhance the effect of spin-orbit coupling at metal/insulator interfaces without using heavy elements.
Magneto-optical spectroscopy based on the transverse magneto-optical Kerr effect (TMOKE) is a sensitive method for investigation of magnetically-ordered media. However, in magnetic materials the optical transitions are usually characterized by spectr
We have performed a systematic magneto-optical Kerr spectroscopy study of GaMnAs with varying Mn densities as a function of temperature, magnetic field, and photon energy. Unlike previous studies, the magnetization easy axis was perpendicular to the
Antiferromagnetic metals attract tremendous interest for memory applications due to their expected fast response dynamics in the terahertz frequency regime. Reading from and writing information into these materials is not easily achievable using magn
We report the engineering of the polar magnetooptical (MO) Kerr effect in perpendicularly magnetized L10-MnAl epitaxial films with remarkably tuned magnetization, strain, and structural disorder by varying substrate temperature (Ts) during molecular-
We have studied the propagation characteristics of spin wave modes in a permalloy stripe by time-resolved magneto-optical Kerr effect techniques. We observe a beating interference pattern in the time domain under the influence of an electrical square