ترغب بنشر مسار تعليمي؟ اضغط هنا

Discovery of two-dimensional Dirac nodal line fermions in monolayer Cu2Si

77   0   0.0 ( 0 )
 نشر من قبل Baojie Feng
 تاريخ النشر 2016
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Topological nodal line semimetals, a novel quantum state of materials, possess topologically nontrivial valence and conduction bands that touch at a line near the Fermi level. The exotic band structure can lead to various novel properties, such as long-range Coulomb interaction and flat Landau levels. Recently, topological nodal lines have been observed in several bulk materials, such as PtSn4, ZrSiS, TlTaSe2 and PbTaSe2. However, in two-dimensional materials, experimental research on nodal line fermions is still lacking. Here, we report the discovery of two-dimensional Dirac nodal line fermions in monolayer Cu2Si based on combined theoretical calculations and angle-resolved photoemission spectroscopy measurements. The Dirac nodal lines in Cu2Si form two concentric loops centred around the {Gamma} point and are protected by mirror reflection symmetry. Our results establish Cu2Si as a new platform to study the novel physical properties in two-dimensional Dirac materials and provide new opportunities to realize high-speed low-dissipation devices.

قيم البحث

اقرأ أيضاً

106 - Si Li , Ying Liu , Zhi-Ming Yu 2019
Dirac point in two-dimensional (2D) materials has been a fascinating subject of research. Recently, it has been theoretically predicted that Dirac point may also be stabilized in 2D magnetic systems. However, it remains a challenge to identify concre te 2D materials which host such magnetic Dirac point. Here, based on first-principles calculations and theoretical analysis, we propose a stable 2D material, the monolayers TaCoTe$_2$, as an antiferromagnetic (AFM) 2D Dirac material. We show that it has an AFM ground state with an out-of-plane N{e}el vector. It hosts a pair of 2D AFM Dirac points on the Fermi level in the absence of spin-orbit coupling (SOC). When the SOC is considered, a small gap is opened at the original Dirac points. Meanwhile, another pair of Dirac points appear on the Brillouin zone boundary below the Fermi level, which are robust under SOC and have a type-II dispersion. Such a type-II AFM Dirac point has not been observed before. We further show that the location of this Dirac point as well as its dispersion type can be controlled by tuning the N{e}el vector orientation.
Dirac nodal line semimetals (DNLSs) host relativistic quasiparticles in their one-dimensional (1D) Dirac nodal line (DNL) bands that are protected by certain crystalline symmetries. Their novel low-energy fermion quasiparticle excitations and transpo rt properties invite studies of relativistic physics in the solid state where their linearly dispersing Dirac bands cross at continuous lines with four-fold degeneracy. In materials studied up to now, the four-fold degeneracy, however, has been vulnerable to suppression by the ubiquitous spin-orbit coupling (SOC). Despite the current effort to discover 3D DNLSs that are robust to SOC by theory, positive experimental evidence is yet to emerge. In 2D DNLSs, because of the decreased total density of states as compared with their 3D counterparts, it is anticipated that their physical properties would be dominated by the electronic states defined by the DNL. It has been even more challenging, however, to discover robust 2D DNLSs against SOC because of their lowered symmetry; no such materials have yet been predicted by theory. By combining molecular beam epitaxy growth, STM, nc-AFM characterisation, with DFT calculations and space group theory analysis, here we reveal a novel class of 2D crystalline DNLSs that host the exact symmetry that protects them against SOC. The discovered quantum material is a brick phase 3-AL Bi(110), whose symmetry protection and thermal stability are imparted by the compressive vdW epitaxial growth on black phosphorus substrates. The BP substrate templates the growth of 3-AL Bi(110) nano-islands in a non-symmorphic space group structure. This crystalline symmetry protects the DNL electronic phase against SOC independent of any orbital or elemental factors. We theoretically establish that this intrinsic symmetry imparts a general, robust protection of DNL in a series of isostructural 2D quantum materials.
Nodal line semimetals in two-dimensional (2-D) materials have attracted intense attention currently. From fundamental physics and spintronic applications points of view, high Curie temperature ferromagnetic (FM) ones with nodal lines robust against s pin-orbit coupling (SOC) are significantly in desirable. Here, we propose that FM K2N monolayer is such Weyl nodal line semimetal. We show that K2N monolayer is dynamically stable, and has a FM ground magnetic state with the out-of-plane [001] magnetization. It shows two nodal lines in the low-energy band structures. Both nodal lines are robust against SOC, under the protection of mirror symmetry. We construct an effective Hamiltonian, which can well characterize the nodal lines in the system. Remarkably, the nodal line semimetal proposed here is distinct from the previously studied ones in that K2N monolayer is 2-D d0-type ferromagnet with the magnetism arising from the partially filled N-p orbitals, which can bring special advantages in spintronic applications. Besides, the Curie temperature in K2N monolayer is estimated to be 942K, being significantly higher than previous FM nodal lines materials. We also find that, specific tensile strains can transform the nodal line from type-I to a type-II one, making its nodal line characteristics even more interesting.
354 - C. Kamal 2019
We predict from DFT based electronic structure calculations that a monolayer made up of Carbon and Arsenic atoms, with a chemical composition (CAs3) forms an energetically and dynamically stable system. The optimized geometry of the monolayer is slig htly different from the buckled geometric configuration observed for silicene and germanene. The results of electronic structure calculations predict that it is a semi-metal. Interestingly, the electronic band structure of this material possesses a linear dispersion and a Dirac cone at the Fermi level around the high symmetric K point in the reciprocal lattice. Thus, at low energy excitation (up to 105 meV), the charge carriers in this system behave as massless Dirac-Fermions. Detailed analysis of partial density of state suggests that the 2pz orbital of C atoms plays vital role in determining the nature of the states, which has a linear dispersion and hence the Dirac cone, around the Fermi level. Thus, the electronic properties of CAs3 monolayer are similar to those of graphene and other group IV based monolayers. In addition, we have also investigated the influence of mechanical strain on the properties of CAs3 monolayer. The buckled configuration becomes the planar configuration for a tensile strain beyond 18%. Our results indicate that the monolayer possesses linear dispersion in the electronic band structure for a wide range of mechanical strain from -12 to 20%, though the position of Dirac point may not lie exactly at the Fermi level. The linear dispersion disappears for a compressive strain beyond -12% & it is due to the drastic changes in the geometrical environment around C atom. Finally, we wish to point out that CAs3 monolayer belongs to the class of Dirac materials where the behaviour of particles, at low energy excitations, are characterized by the Dirac-like Hamiltonian rather than the Schrodinger Hamiltonian.
Based on first-principles calculations, we predict a new two-dimensional ferromagnetic material that exhibits exotic Fermi surface topology. We show that monolayer hexagonal indium carbide ({em h}-InC) is thermodynamically and dynamically stable, and it energetically favors the ferromagnetic ordering of spins. The perfectly planar geometry in two dimensions, together with ferromagnetism, gives rise to a unique opportunity to encounter intriguing electronic properties, captured in the Fermi surface and band topology. We show that multiple nodal lines coexist in momentum space, accompanied by the electron and hole pockets that touch each other linearly at the nodal lines. Inclusion of spin-orbit coupling enriches the magnetic and electronic properties of {em h}-InC. Spin-orbit coupling leads to an easy-plane type magnetocrystalline anisotropy, and the nodal lines can be tuned into topological nodal points, contingent upon the magnetization direction. Symmetry analysis and a tight-binding model are provided to explain the nodal structure of the bands. Our findings suggest {em h}-InC as a new venue for supporting carbon-based magnetism and exotic band topology in two dimensions.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا