اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدSuperconductivity emerging from an electronic phase separation in the charge ordered phase of RbFe$_2$As$_2$
69
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
$^{75}$As, $^{87}$Rb and $^{85}$Rb nuclear quadrupole resonance (NQR) and $^{87}$Rb nuclear magnetic resonance (NMR) measurements in RbFe$_2$As$_2$ iron-based superconductor are presented. We observe a marked broadening of $^{75}$As NQR spectrum below $T_0simeq 140$ K which is associated with the onset of a charge order in the FeAs planes. Below $T_0$ we observe a power-law decrease in $^{75}$As nuclear spin-lattice relaxation rate down to $T^*simeq 20$ K. Below that temperature the nuclei start to probe different dynamics owing to the different local electronic configurations induced by the charge order. A fraction of the nuclei probes spin dynamics associated with electrons approaching a localization while another fraction probes activated dynamics possibly associated with a pseudogap. These different trends are discussed in the light of an orbital selective behaviour expected for the electronic correlations.
قيم البحث
اقرأ أيضاً
We investigated the transport properties of BaFe$_2$As$_2$ single crystals before and after annealing with BaAs powder. The annealing remarkably improves transport properties, in particular the magnitude of residual resistivity which decreases by a f
actor of more than 10. From the resistivity measurement on detwinned crystals we found that the anisotropy of the in-plane resistivity is remarkably diminished after annealing, indicative of dominant contributions to the charge transport from the carriers with isotropic and high mobility below magnetostructural transition temperature $T_{rm s}$ and the absence of nematic state above $T_{rm s}$. We found that the Hall resistivity shows strong non-linearity against magnetic field and the magnetoresistance becomes very large at low temperatures. These results give evidence for the manifestation of multiple carriers with distinct characters in the ordered phase below $T_{rm s}$. By analyzing the magnetic field dependences, we found that at least three carriers equally contribute to the charge transport in the ordered phase, which is in good agreement with the results of recent quantum oscillation measurements.
The recent discovery of pressure induced superconductivity in the binary helimagnet CrAs has attracted much attention. How superconductivity emerges from the magnetic state and what is the mechanism of the superconducting pairing are two important is
sues which need to be resolved. In the present work, the suppression of magnetism and the occurrence of superconductivity in CrAs as a function of pressure ($p$) were studied by means of muon spin rotation. The magnetism remains bulk up to $psimeq3.5$~kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at $psimeq$7~kbar. At 3.5 kbar superconductivity abruptly appears with its maximum $T_c simeq 1.2$~K which decreases upon increasing the pressure. In the intermediate pressure region ($3.5lesssim plesssim 7$~kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature ($T_c$) and of the superfluid density ($rho_s$). A scaling of $rho_s$ with $T_c^{3.2}$ as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs.
We present magnetic susceptibility and electrical transport measurements of the highly anisotropic compound LaSb$_2$ observing a very broad transition into a clean, consistent with type-I, superconducting state with distinct features of 2 dimensional
ity. Application of hydrostatic pressure induces a 2- to 3-dimensional crossover evidenced by a reduced anisotropy and transition width. The superconducting transition appears phase fluctuation limited at ambient pressure with fluctuations observed for temperatures greater than 8 times the superconducting critical temperature.
We report the effect of applied pressures on magnetic and superconducting order in single crystals of the aliovalent La-doped iron pnictide material Ca$_{1-x}$La$_{x}$Fe$_{2}$As$_{2}$. Using electrical transport, elastic neutron scattering and resona
nt tunnel diode oscillator measurements on samples under both quasi-hydrostatic and hydrostatic pressure conditions, we report a series of phase diagrams spanning the range of substitution concentrations for both antiferromagnetic and superconducting ground states that include pressure-tuning through the antiferromagnetic (AFM) quantum critical point. Our results indicate that the observed superconducting phase with maximum transition temperature of $T_{c}$=47 K is intrinsic to these materials, appearing only upon suppression of magnetic order by pressure tuning through the AFM critical point. In contrast to all other intermetallic iron-pnictide superconductors with the ThCr$_2$Si$_2$ structure, this superconducting phase appears to exist only exclusively from the antiferromagnetic phase in a manner similar to the oxygen- and fluorine-based iron-pnictide superconductors with the highest transition temperatures reported to date. The unusual dichotomy between lower-$T_{c}$ systems with coexistent superconductivity and magnetism and the tendency for the highest-$T_{c}$ systems to show non-coexistence provides an important insight into the distinct transition temperature limits in different members of the iron-based superconductor family.
We report synthesis, crystal structure and physical properties of a quinary iron-arsenide fluoride KCa$_2$Fe$_4$As$_4$F$_2$. The new compound crystallizes in a body-centered tetragonal lattice (with space group $I4/mmm$, $a$ = 3.8684(2) {AA}, c = 31.
007(1) {AA}, and $Z$ = 2), which contains double Fe$_2$As$_2$ conducting layers separated by insulating Ca$_2$F$_2$ layers. Our measurements of electrical resistivity, dc magnetic susceptibility and heat capacity demonstrate bulk superconductivity at 33 K in KCa$_2$Fe$_4$As$_4$F$_2$.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
