ترغب بنشر مسار تعليمي؟ اضغط هنا

Magnetism of the antiferromagnetic spin-$frac{1}{2}$ tetramer compound CuInVO$_5$

129   0   0.0 ( 0 )
 نشر من قبل Masashi Hase
 تاريخ النشر 2016
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We measured the temperature dependence of the magnetic susceptibility and specific heat and the magnetic-field dependence of the magnetization of CuInVO$_5$. An antiferromagnetically ordered state appears below $T_{rm N} = 2.7$ K. We observed a $frac{1}{2}$ quantum magnetization plateau above 30 T at 1.3 K. We show that the spin system consists of antiferromagnetic spin-$frac{1}{2}$ tetramers with $J_1 = 240 pm 20$ and $J_2 = -142 pm 10$ K for the intratetramer interactions.



قيم البحث

اقرأ أيضاً

We measured magnetization, specific heat, electron spin resonance, neutron diffraction, and inelastic neutron scattering of CrVMoO$_7$ powder. An antiferromagnetically ordered state appears below $T_{rm N} = 26.5 pm 0.8$ K. We consider that the proba ble spin model for CrVMoO$_7$ is an interacting antiferromagnetic spin-$frac{3}{2}$ dimer model. We evaluated the intradimer interaction $J$ to be $25 pm 1$ K and the effective interdimer interaction $J_{rm eff}$ to be $8.8 pm 1$ K. CrVMoO$_7$ is a rare spin dimer compound that shows an antiferromagnetically ordered state at atmospheric pressure and zero magnetic field. The magnitude of ordered moments is $0.73(2) mu_{rm B}$. It is much smaller than a classical value $sim 3 mu_{rm B}$. Longitudinal-mode magnetic excitations may be observable in single crystalline CrVMoO$_7$.
Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$frac{1}{2}$ state due to the combined effect of crystal electric field and spin orbit coupl ing. Magnetic susceptibility measurements and $^7$Li nuclear magnetic resonance experiments reveal the absence of magnetic long range ordering down to 2~K, which suggests a possible quantum spin liquid ground state. A dominant antiferromagnetic nearest neighbour exchange interaction $J/k_{rm B}simeq$ 5.3~K could be extracted form the magnetic susceptibility. The NMR linewidth analysis yields the coupling constant between the Li nuclei and Yb$^{3+}$ ions which was found to be purely dipolar in nature.
We report zero and longitudinal magnetic field muon spin relaxation measurements of the spin S=1/2 antiferromagnetic Heisenberg chain material SrCuO2. We find that in a weak applied magnetic field B the spin-lattice relaxation rate follows a power la w B^n with n=-0.9(3). This result is temperature independent for 5K < T < 300 K. Within conformal field theory and using the Muller ansatz we conclude ballistic spin transport in SrCuO2.
562 - B. Y. Pan , Y. Wang , L. J. Zhang 2013
Single crystals of a metal organic complex ce{(C5H12N)CuBr3} (ce{C5H12N} = piperidinium, pipH for short) have been synthesized and the structure was determined by single-crystal X-ray diffraction. ce{(pipH)CuBr3} crystallizes in the monoclinic group $C$2/$c$. Edging-sharing ce{CuBr5} units link to form zigzag chains along the $c$ axis and the neighboring Cu(II) ions with spin-1/2 are bridged by bi-bromide ions. Magnetic susceptibility data down to 1.8 K can be well fitted by the Bonner-Fisher formula for antiferromagnetic spin-1/2 chain, giving the intrachain magnetic coupling constant $J$ $sim$ 17 K. At zero field, ce{(pipH)CuBr3} shows three-dimensional (3D) order below $T_N$ = 1.68 K. Calculated by the mean-field theory, the interchain coupling constant $J$ = 0.65 K is obtained and the ordered magnetic moment $m_0$ is about 0.20 $mu_B$. This value of $m_0$ makes ce{(pipH)CuBr3} a rare compound suitable to study the dimensional crossover problem in magnetism, since both 3D order and one-dimensional (1D) quantum fluctuations are prominent. In addition, specific heat measurements reveal two successive magnetic transitions with lowering temperature when external field $H geq$ 3 T is applied along the $a$ axis. The $H$ - $T$ phase diagram of ce{(pipH)CuBr3} is roughly constructed. The interplay between exchange interactions, dimensionality, Zeeman energy and possible Dzyaloshinkii-Moriya interaction should be the driving force for the multiple phase transitions.
238 - P. H. Y. Li , R. F. Bishop 2018
The zero-temperature quantum phase diagram of the spin-$frac{1}{2}$ $J_{1}$--$J_{2}$--$J_{1}^{perp}$ model on an $AA$-stacked bilayer honeycomb lattice is investigated using the coupled cluster method (CCM). The model comprises two monolayers in each of which the spins, residing on honeycomb-lattice sites, interact via both nearest-neighbor (NN) and frustrating next-nearest-neighbor isotropic antiferromagnetic (AFM) Heisenberg exchange iteractions, with respective strengths $J_{1} > 0$ and $J_{2} equiv kappa J_{1}>0$. The two layers are coupled via a comparable Heisenberg exchange interaction between NN interlayer pairs, with a strength $J_{1}^{perp} equiv delta J_{1}$. The complete phase boundaries of two quasiclassical collinear AFM phases, namely the N{e}el and N{e}el-II phases, are calculated in the $kappa delta$ half-plane with $kappa > 0$. Whereas on each monolayer in the N{e}el state all NN pairs of spins are antiparallel, in the N{e}el-II state NN pairs of spins on zigzag chains along one of the three equivalent honeycomb-lattice directions are antiparallel, while NN interchain spins are parallel. We calculate directly in the thermodynamic (infinite-lattice) limit both the magnetic order parameter $M$ and the excitation energy $Delta$ from the $s^{z}_{T}=0$ ground state to the lowest-lying $|s^{z}_{T}|=1$ excited state (where $s^{z}_{T}$ is the total $z$ component of spin for the system as a whole, and where the collinear ordering lies along the $z$ direction) for both quasiclassical states used (separately) as the CCM model state, on top of which the multispin quantum correlations are then calculated to high orders ($n leq 10$) in a systematic series of approximations involving $n$-spin clusters. The sole approximation made is then to extrapolate the sequences of $n$th-order results for $M$ and $Delta$ to the exact limit, $n to infty$.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا