ترغب بنشر مسار تعليمي؟ اضغط هنا

Anomalous Brownian motion of colloidal particle in a nematic environment: effect of the director fluctuations

199   0   0.0 ( 0 )
 نشر من قبل T. Turiv
 تاريخ النشر 2015
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

As recently reported [Turiv T. et al., Science, 2013, Vol. 342, 1351], fluctuations in the orientation of the liquid crystal (LC) director can transfer momentum from the LC to a colloid, such that the diffusion of the colloid becomes anomalous on a short time scale. Using video microscopy and single particle tracking, we investigate random thermal motion of colloidal particles in a nematic liquid crystal for the time scales shorter than the expected time of director fluctuations. At long times, compared to the characteristic time of the nematic director relaxation we observe typical anisotropic Brownian motion with the mean square displacement (MSD) linear in time $tau$ and inversly proportional to the effective viscosity of the nematic medium. At shorter times, however, the dynamics is markedly nonlinear with MSD growing more slowly (subdiffusion) or faster (superdiffusion) than $tau$. These results are discussed in the context of coupling of colloidal particles dynamics to the director fluctuation dynamics.



قيم البحث

اقرأ أيضاً

159 - R. Tsekov 2017
The Klein-Kramers equation, governing the Brownian motion of a classical particle in quantum environment under the action of an arbitrary external potential, is derived. Quantum temperature and friction operators are introduced and at large friction the corresponding Smoluchowski equation is obtained. Introducing the Bohm quantum potential, this Smoluchowski equation is extended to describe the Brownian motion of a quantum particle in quantum environment.
The analytical expressions for the time-dependent cross-correlations of the translational and rotational Brownian displacements of a particle with arbitrary shape are derived. The reference center is arbitrary, and the reference frame is such that th e rotational-rotational diffusion tensor is diagonal.
The director configuration of disclination lines in nematic liquid crystals in the presence of an external magnetic field is evaluated. Our method is a combination of a polynomial expansion for the director and of further analytical approximations wh ich are tested against a numerical shooting method. The results are particularly simple when the elastic constants are equal, but we discuss the general case of elastic anisotropy. The director field is continuous everywhere apart from a straight line segment whose length depends on the value of the magnetic field. This indicates the possibility of an elongated defect core for disclination lines in nematics due to an external magnetic field.
The nematic ordering in semiflexible polymers with contour length $L$ exceeding their persistence length $ell_p$ is described by a confinement of the polymers in a cylinder of radius $r_{eff}$ much larger than the radius $r_rho$, expected from the re spective concentration of the solution. Large scale Molecular Dynamics simulations combined with Density Functional Theory are used to locate the Isotropic-Nematic ($I-N$)-transition and to validate this cylindrical confinement. Anomalous fluctuations, due to chain deflections from neighboring chains in the nematic phase are proposed. Considering deflections as collective excitations in the nematically ordered phase of semiflexible polymers elucidates the origins of shortcomings in the description of the $I-N$ transition by existing theories.
108 - J.T. Padding , A.A. Louis 2007
We apply a hybrid Molecular Dynamics and mesoscopic simulation technique to study the steady-state sedimentation of hard sphere particles for Peclet numbers (Pe) ranging from 0.08 to 12. Hydrodynamic back-flow causes a reduction of the average sedime ntation velocity relative to the Stokes velocity. We find that this effect is independent of Pe number. Velocity fluctuations show the expected effects of thermal fluctuations at short correlation times. At longer times, non-equilibrium hydrodynamic fluctuations are visible, and their character appears to be independent of the thermal fluctuations. The hydrodynamic fluctuations dominate the diffusive behavior even for modest Pe number, while conversely the short-time fluctuations are dominated by thermal effects for a surprisingly large Pe numbers. Inspired by recent experiments, we also study finite sedimentation in a horizontal planar slit. In our simulations distinct lateral patterns emerge, in agreement with observations in the experiments.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا