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A hierarchical multiscale approach to model the magnetization dynamics of ferromagnetic ran- dom alloys is presented. First-principles calculations of the Heisenberg exchange integrals are linked to atomistic spin models based upon the stochastic Landau-Lifshitz-Gilbert (LLG) equation to calculate temperature-dependent parameters (e.g., effective exchange interactions, damping param- eters). These parameters are subsequently used in the Landau-Lifshitz-Bloch (LLB) model for multi-sublattice magnets to calculate numerically and analytically the ultrafast demagnetization times. The developed multiscale method is applied here to FeNi (permalloy) as well as to copper- doped FeNi alloys. We find that after an ultrafast heat pulse the Ni sublattice demagnetizes faster than the Fe sublattice for the here-studied FeNi-based alloys.
Element specific ultrafast demagnetization was studied in Fe$_{1-x}$Ni$_{x}$ alloys, covering the concentration range between $0.1<x<0.9$. For all compositions, we observe a delay in the onset of Ni demagnetization relative to the Fe demagnetization.
Recent investigations have advanced the understanding of how structure-property relationships in ferromagnetic metal alloys affect the magnetization dynamics on nanosecond time-scales. A similar understanding for magnetization dynamics on femto- to p
We provide a model for the prediction of the electronic and magnetic configurations of ferromagnetic Fe after an ultrafast decrease or increase of magnetization. The model is based on the well-grounded assumption that, after the ultrafast magnetizati
Polyelectrolyte gels are a very attractive class of actuation materials with remarkable electronic and mechanical properties with a great similarity to biological contractile tissues. They consist of a polymer network with ionizable groups and a liqu
Identifying an efficient pathway to change the order parameter via a subtle excitation of the coupled high-frequency mode is the ultimate goal of the field of ultrafast phase transitions. This is an especially interesting research direction in magnet