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تسجيل مستخدم جديدEnhancement of Light Yield and Stability of Radio-Pure Tetraphenyl-Butadiene Based Coatings for VUV Light Detection in Cryogenic Environments
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The detection of VUV scintillation light, e.g. in (liquid) argon detectors, commonly includes a reflector with a fluorescent coating, converting UV photons to visible light. The light yield of these detectors depends directly on the conversion efficiency. Several coating/reflector combinations were produced using VM2000, a specular reflecting multi layer polymer, and Tetratex, a diffuse reflecting PTFE fabric, as reflector foils. The light yield of these coatings was optimised and has been measured in a dedicated liquid argon setup built at the University of Zurich. It employs a small, 1.3 kg LAr cell viewed by a 3-inch, low radioactivity PMT of type R11065-10 from Hamamatsu. The cryogenic stability of these coatings was additionally studied. The optimum reflector/coating combination was found to be Tetratex dip coated with Tetraphenyl-butadiene with a thickness of 0.9 mg/cm$^2$ resulting in a 3.6 times higher light yield compared to uncoated VM2000. Its performance was stable in long term measurements, ran up to 100 days, in liquid argon. This coated reflector was further investigated concerning radioactive impurities found to be suitable for current and upcoming low-background experiments. Therefore it is used for the liquid argon veto in Phase II of the GERDA neutrinoless double beta decay experiment.
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We report on studies of degradation mechanisms of tetraphenyl butadiene (TPB) coatings of the type used in neutrino and dark matter liquid argon experiments. Using gas chromatography coupled to mass spectrometry we have detected the ultraviolet-block
ing impurity benzophenone (BP). We monitored the drop in performance and increase of benzophenone concentration in TPB plates with exposure to ultraviolet (UV) light, and demonstrate the correlation between these two variables. Based on the presence and initially exponential increase in the concentration of benzophenone observed, we propose that TPB degradation is a free radical-mediated photooxidation reaction, which is subsequently confirmed by displaying delayed degradation using a free radical inhibitor. Finally we show that the performance of wavelength-shifting coatings of the type envisioned for the LBNE experiment can be improved by 10-20%, with significantly delayed UV degradation, by using a 20% admixture of 4-tert-Butylcatechol.
To increase the light yield of a liquid Ar (LAr) detector, we optimized the evaporation technique of tetraphenyl butadiene (TPB) on the detector surface and tested the operability of a silicon photomultiplier (SiPM), namely, the multi-pixel photon co
unter with through-silicon-via (TSV-MPPC, Hamamatsu Photonics K.K.) at LAr temperature. TPB converts the LAr scintillations (vacuum ultraviolet light) to visible light, which can be detected by high-sensitivity photosensors. Because the light yield depends on the deposition mass of TPB on the inner surface of the detector, we constructed a well-controlled TPB evaporator to ensure reproducibility and measured the TPB deposition mass using a quartz crystal microbalance sensor. After optimizing the deposition mass of TPB (30 $mu g/cm^2$ on the photosensor window and 40 $mu g/cm^2$ on the detector wall), the light yield was 12.8 $pm$ 0.3 p.e./keVee using PMTs with a quantum efficiency of approximately 30% for TPB-converted light. We also tested the low-temperature tolerance of TSV-MPPC, which has a high photon-detection efficiency, in the LAr environment. The TSV-MPPC detected the LAr scintillations converted by TPB with a photon-detection efficiency exceeding 50%.
TetraPhenyl Butadiene is the wavelength shifter most widely used in combination with liquid Argon. The latter emits scintillation photons with a wavelength of 127 nm that need to be downshifted to be detected by photomultipliers with glass or quartz
windows. TetraPhenyl Butadiene has been demonstrated to have an extremely high conversion efficiency, possibly higher than 100 % for 127 nm photons, while there is no precise information about the time dependence of its emission. It is usually assumed to be exponentially decaying with a characteristic time of the order of one ns, as an extrapolation from measurements with exciting radiation in the near UV. This work shows that TetraPhenyl Butadiene, when excited by 127 nm photons, reemits photons not only with a very short decay time, but also with slower ones due to triplet states de-excitations. This fact can strongly contribute to clarify the anomalies in liquid Argon scintillation light reported in literature since seventies, namely the inconsistency in the measured values of the long decay time constant and the appearance of an intermediate component. Similar effects should be also expected when the TPB is used in combination with Helium and Neon, that emit scintillation photons with wavelengths shorter than 127 nm.
We study the stability of three types of popularly employed TPB coatings under immersion in liquid argon. TPB emanation from each coating is quantified by fluorescence assay of molecular sieve filter material after a prolonged soak time. Two of the c
oatings are shown to emanate a detectable concentration of TPB into argon over a 24 hour period, which corresponds to tens of parts per billion in argon by mass. In an independent setup, the dissolved or suspended TPB is shown to produce a wavelength shifting effect in the argon bulk. Interpretations of these results and implications for present and future liquid argon time projection chamber experiments are discussed.
Acrylic (poly(methyl methacrylate) or PMMA) is commonly used as a vessel to hold scintillating liquids in rare-event searches. Certain types of PMMA can fluoresce with a low efficiency at room temperature. We have investigated the fluorescence spectr
a under 280nm ultraviolet (UV) excitation of the PMMA used in the DEAP dark matter search at various low temperatures. Fluorescence of this PMMA is observed, with an increasing intensity as the sample is cooled from a temperature of 300K down to 4K. The common wavelength-shifter tetraphenyl butadiene (TPB) is also measured for use as a reference.
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