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We have identified a novel phase stability mechanism from the intracavity field-induced self-organization of a fast-moving molecular beam into travelling molecular packets in the bad cavity regime, which is then used to decelerate the molecular packets by feedback-controlled time-varying laser pumps to the cavity. We first applied the linear stability analysis to derive an expression for this self-organization in the adiabatic limit and show that the self-organization of the beam leads to the formation of travelling molecular packets, which in turn function as a dynamic Bragg grating, thus modulating periodically the intracavity field by superradiant scattering of the pump photons. The modulation encodes the position information of the molecular packets into the output of the intracavity field instantaneously. We then applied time-varying laser pumps that are automatically switched by the output of the intracavity field to slow down the molecular packets via a feedback mechanism and found that most of the molecules in the molecular packets are decelerated to zero central velocity after tens of stages. Our cavity-based deceleration proposal works well in the bad cavity regime, which is very different from the conventional cavity- based cooling strategies where a good cavity is preferred. Practical issues in realizing the proposal are also discussed.
Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few milliseconds
We present an experimental study of cavity assisted Rydberg atom electromagnetically induced transparency (EIT) using a high-finesse optical cavity ($F sim 28000$). Rydberg atoms are excited via a two-photon transition in a ladder-type EIT configurat
The residual cavity-pulling effect limits further narrowing of linewidth in dual-wavelength (DW) good-bad-cavity active optical clocks (AOCs). In this paper, we for the first time experimentally realize the cavity-length stabilization of the 1064/147
We propose a method to exploit high finesse optical resonators for light assisted coherent manipulation of atomic ensembles, overcoming the limit imposed by the finite response time of the cavity. The key element of our scheme is to rapidly switch th
Heavy diatomic molecules have been identified as good candidates for use in electron electric dipole moment (eEDM) searches. Suitable molecular species can be produced in pulsed beams, but with a total flux and/or temporal evolution that varies signi