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Enriched Zn$^{100}$MoO$_4$ scintillating bolometers to search for $0 u 2beta$ decay of $^{100}$Mo with the LUMINEU experiment

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 نشر من قبل Andrea Giuliani
 تاريخ النشر 2014
  مجال البحث فيزياء
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The LUMINEU project aims at performing a demonstrator underground experiment searching for the neutrinoless double beta decay of the isotope $^{100}$Mo embedded in zinc molybdate (ZnMoO$_4$) scintillating bolometers. In this context, a zinc molybdate crystal boule enriched in $^{100}$Mo to 99.5% with a mass of 171 g was grown for the first time by the low-thermal-gradient Czochralski technique. The production cycle provided a high yield (the crystal boule mass was 84% of initial charge) and an acceptable level -- around 4% -- of irrecoverable losses of the costy enriched material. Two crystals of 59 g and 63 g, obtained from the enriched boule, were tested aboveground at milli-Kelvin temperature as scintillating bolometers. They showed a high detection performance, equivalent to that of previously developed natural ZnMoO$_4$ detectors. These results pave the way to future sensitive searches based on the LUMINEU technology, capable to approach and explore the inverted hierarchy region of the neutrino mass pattern.



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The technology of scintillating bolometers based on zinc molybdate (ZnMoO$_4$) crystals is under development within the LUMINEU project to search for 0$ u$2$beta$ decay of $^{100}$Mo with the goal to set the basis for large scale experiments capable to explore the inverted hierarchy region of the neutrino mass pattern. Advanced ZnMoO$_4$ crystal scintillators with mass of $sim$~0.3 kg were developed and Zn$^{100}$MoO$_4$ crystal from enriched $^{100}$Mo was produced for the first time by using the low-thermal-gradient Czochralski technique. One ZnMoO$_4$ scintillator and two samples (59 g and 63 g) cut from the enriched boule were tested aboveground at milli-Kelvin temperature as scintillating bolometers showing a high detection performance. The first results of the low background measurements with three ZnMoO$_4$ and two enriched detectors installed in the EDELWEISS set-up at the Modane Underground Laboratory (France) are presented.
This paper reports on the development of a technology involving $^{100}$Mo-enriched scintillating bolometers, compatible with the goals of CUPID, a proposed next-generation bolometric experiment to search for neutrinoless double-beta decay. Large mas s ($sim$1~kg), high optical quality, radiopure $^{100}$Mo-containing zinc and lithium molybdate crystals have been produced and used to develop high performance single detector modules based on 0.2--0.4~kg scintillating bolometers. In particular, the energy resolution of the lithium molybdate detectors near the $Q$-value of the double-beta transition of $^{100}$Mo (3034~keV) is 4--6~keV FWHM. The rejection of the $alpha$-induced dominant background above 2.6~MeV is better than 8$sigma$. Less than 10~$mu$Bq/kg activity of $^{232}$Th ($^{228}$Th) and $^{226}$Ra in the crystals is ensured by boule recrystallization. The potential of $^{100}$Mo-enriched scintillating bolometers to perform high sensitivity double-beta decay searches has been demonstrated with only 10~kg$times$d exposure: the two neutrino double-beta decay half-life of $^{100}$Mo has been measured with the up-to-date highest accuracy as $T_{1/2}$ = [6.90 $pm$ 0.15(stat.) $pm$ 0.37(syst.)] $times$ 10$^{18}$~yr. Both crystallization and detector technologies favor lithium molybdate, which has been selected for the ongoing construction of the CUPID-0/Mo demonstrator, containing several kg of $^{100}$Mo.
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