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تسجيل مستخدم جديدInterface superconductivity: History, development and prospects
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The concept of interface superconductivity was introduced over 50 years ago. Some of the greatest physicists of that time wondered whether a quasi-two-dimensional (2D) superconductor can actually exist, what are the peculiarities of 2D superconductivity, and how does the reduced dimensionality affect the critical temperature (Tc). The discovery of high-temperature superconductors, which are composed of coupled 2D superconducting layers, further increased the interest in reduced dimensionality structures. In parallel, the advances in experimental techniques made it possible to grow epitaxial 2D structures with atomically flat surfaces and interfaces, enabling some of the experiments that were proposed decades ago to be performed finally. Now we know that interface superconductivity can occur at the junction of two different materials (metals, insulators, semiconductors). This phenomenon is being explored intensely; it is also exploited as a means to increase Tc or to study quantum critical phenomena. This research may or may not produce a superconductor with a higher Tc or a useful superconducting electronic device but it will likely bring in new insights into the physics underlying high-temperature superconductivity.
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The interface superconductivity in LaAlO$_{3}$-SrTiO$_{3}$ heterostructures reveals a non-monotonic behavior of the critical temperature as a function of the two-dimensional density of charge carriers. We develop a theoretical description of interfac
e superconductivity in strongly polar heterostructures, based on the dielectric function formalism. The density dependence of the critical temperature is calculated accounting for all phonon branches including different types of optical (interface and half-space) and acoustic phonons. The LO- and acoustic-phonon-mediated electron-electron interaction is shown to be the dominating mechanism governing the superconducting phase transition in the heterostructure.
At interfaces between complex oxides it is possible to generate electronic systems with unusual electronic properties, which are not present in the isolated oxides. One important example is the appearance of superconductivity at the interface between
insulating oxides, although, until now, with very low Tc. We report the occurrence of high Tc superconductivity in the bilayer CaCuO2/SrTiO3, where both the constituent oxides are insulating. In order to obtain a superconducting state, the CaCuO2/SrTiO3 interface must be realized between the Ca plane of CaCuO2 and the TiO2 plane of SrTiO3. Only in this case extra oxygen ions can be incorporated in the interface Ca plane, acting as apical oxygen for Cu and providing holes to the CuO2 planes. A detailed hole doping spatial profile has been obtained by STEM/EELS at the O K-edge, clearly showing that the (super)conductivity is confined to about 1-2 CaCuO2 unit cells close to the interface with SrTiO3. The results obtained for the CaCuO2/SrTiO3 interface can be extended to multilayered high Tc cuprates, contributing to explain the dependence of Tc on the number of CuO2 planes in these systems.
LaAlO3 and SrTiO3 are insulating, nonmagnetic oxides, yet the interface between them exhibits a two-dimensional electron system with high electron mobility,1 superconductivity at low temperatures,2-6 and electric-field-tuned metal-insulator and super
conductorinsulator phase transitions.3,6-8 Bulk magnetization and magnetoresistance measurements also suggest some form of magnetism depending on preparation conditions5,9-11 and suggest a tendency towards nanoscale electronic phase separation.10 Here we use local imaging of the magnetization and magnetic susceptibility to directly observe a landscape of ferromagnetism, paramagnetism, and superconductivity. We find submicron patches of ferromagnetism in a uniform background of paramagnetism, with a nonuniform, weak diamagnetic superconducting susceptibility at low temperature. These results demonstrate the existence of nanoscale phase separation as suggested by theoretical predictions based on nearly degenerate interface sub-bands associated with the Ti orbitals.12,13 The magnitude and temperature dependence of the paramagnetic response suggests that the vast majority of the electrons at the interface are localized, and do not contribute to transport measurements.3,6,7 In addition to the implications for magnetism, the existence of a 2D superconductor at an interface with highly broken inversion symmetry and a ferromagnetic landscape in the background suggests the potential for exotic superconducting phenomena.
In polar-oxide interfaces, a certain number of monolayers (ML) is needed for conductivity to appear. This threshold for conductivity is explained by accumulating sufficient electric potential to initiate charge transfer to the interface. Here we stud
y experimentally and theoretically the (111) SrTiO3/LaAlO3 interface where a critical thickness, tc, of nine epitaxial LaAlO3 ML is required to turn the interface from insulating to conducting and even superconducting. We show that tc decreases to 3ML when depositing a cobalt over-layer (capping) and 6ML for platinum capping. The latter result contrasts with the (100) interface, where platinum capping increases tc beyond the bare interface. The observed threshold for conductivity for the bare and the metal-capped interfaces is confirmed by our density functional theory calculations. Interestingly, for (111) SrTiO3/LaAlO3/Metal interfaces, conductivity appears concomitantly with superconductivity in contrast with the (100) SrTiO3/LaAlO3/Metal interfaces where tc is smaller than the critical thickness for superconductivity. We attribute this dissimilarity to the different orbital polarization of eg for the (111) versus dxy for the (001) interface.
Superconductivity (S) and ferromagnetism (F) are probed through transport and magnetization measurements in nanometer scale HoNi$_5$-NbN (F-S) bilayers and HoNi$_5$-NbN-HoNi$_5$ (F-S-F) trilayers. The choice of materials has been made on the basis of
their comparable ordering temperatures and strong magnetic anisotropy in HoNi$_5$. We observe the normal state reentrant behavior in resistance vs. temperature plots of the F-S-F structures just below the superconducting transition in the limited range of HoNi$_5$ layer thickness d$_{HN}$ (20 nm $<$ d$_{HN}$ $<$ 80 nm) when d$_{NbN}$ is fixed at $simeq$ 10 nm. The reentrance is quenched by increasing the out-of-plane (H$_{perp}$) magnetic field and transport current where as in-plane (H$_{parallel}$) field of $leq$ 1500 Oe has no effect on the reentrance. The thermally activated flux flow characteristics of the S, F-S and F-S-F layers reveal a transition from collective pinning to single vortex pinning as we place F layers on both sides of the S film. The origin of the reentrant behavior seen here in the range of 0.74 $leq$ T$_{Curie}$/T$_C$ $leq$ 0.92 is attribute to a delicate balance between the magnetic exchange energy and the condensation energy in the interfacial regions of the trilayer.
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