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We report experiments on the generation of third and fifth harmonics of millijoule-level, tightly focused, femtosecond laser pulses at 2.2 {mu}m wavelength in air. The measured ratio of yields of the third and fifth harmonics in our setup is about 2 cdot 10-4. This result contradicts the recent suggestion that the Kerr effect in air saturates and changes sign in ultra-intense optical fields.
Quantum cascade lasers (QCL) have revolutionized the generation of mid-infrared light. Yet, the ultrafast carrier transport in mid-infrared QCLs has so far constituted a seemingly insurmountable obstacle for the formation of ultrashort light pulses.
We investigate the generation of broadband terahertz (THz) pulses with phase singularity from air plasmas created by fundamental and second harmonic laser pulses. We show that when the second harmonic beam carries a vortex charge, the THz beam acquir
The possibility of performing time-resolved spectroscopic studies in the molecular fingerprinting region or extending the cut-off wavelength of high-harmonic generation has recently boosted the development of efficient mid-infrared ultrafast lasers.
Investigation of laser matter interaction with electromagnetic codes requires to implement sources for the electromagnetic fields. A way to do so is to prescribe the fields at the numerical box boundaries in order to achieve the desired fields inside