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Neutron scattering experiments were performed on single crystals of layered cobalt-oxides La2-xCaxCoO4 (LCCO) to characterize the charge and spin orders in a wide hole-doping range of 0.3<x<0.8. For a commensurate value of x=0.5 in (H,0,L) plane, two types of superlattice reflections concomitantly appear at low temperature; one corresponds to a checkerboard charge ordered pattern of Co2+/Co3+ ions and the other is magnetic in origin. Further, the latter magnetic-superlattice peaks show two types of symmetry in the reflections, suggesting antiferromagnetic-stacking (AF-S) and ferromagnetic-stacking (F-S) patterns of spins along the c direction. From the hole-doping dependence, the in-plane correlation lengths of both charge and spin orders are found to give a maximum at x=0.5. These features are the same with those of x=0.5 in La1-xSr1+xMnO4 (LSMO), a typical checkerboard and spin ordered compound. However, in (H,H,L) plane, we found a magnetic scattering peak at Q=(1/4,1/4,1/2) position below TN. This magnetic peak can not be understood by considering the Co2+ spin configuration, suggesting that this peak is originated from Co3+ spin order. By analyzing these superlattice reflections, we found that they are originated from high-spin state of Co3+ spin order.
Recent experimental discoveries have brought a diverse set of broken symmetry states to the center stage of research on cuprate superconductors. Here, we focus on a thematic understanding of the diverse phenomenology by exploring a strong-coupling me
We investigate the interplay between spin and orbital correlations in monolayer and bilayer manganites using an effective spin-orbital t-J model which treats explicitly the e_g orbital degrees of freedom coupled to classical t_{2g} spins. Using finit
We have performed non-resonant x-ray diffraction, resonant soft and hard x-ray magnetic diffraction, soft x-ray absorption and x-ray magnetic circular dichroism measurements to clarify the electronic and magnetic states of the Co3+ ions in GdBaCo2O5.
In the presence of nonlocal phase shift effects, a quasiparticle can remain topologically stable even in a spin-charge separation state due to the confinement effect introduced by the phase shifts at finite doping. True deconfinement only happens in
We investigate the low temperature magnetic field dependences of both the resistivity and the magnetization in the misfit cobaltate Ca3Co4O9 from 60 K down to 2 K. The measured negative magnetoresistance reveals a scaling behavior with the magnetizat