اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدDirect observation of strong correlations near the band insulator regime of Bi misfit cobaltates
42
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
We present the first angle-resolved photoemission (ARPES) measurement of Fermi Surface in the misfit cobaltate [Bi2Ba2O4].[CoO2]~2. This compound contains the same triangular Co planes as Na cobaltates, but in a different 3D environment. Our data establish the similarity of their electronic structure. We propose that the peculiar lineshape of all cobaltates is of the peak-dip-hump type, due to strong many-body effects. We detect a progressive transfer of spectral weight from the quasiparticle feature near Ef to a broad hump in misfit phases where Ba is replaced by Sr or Ca. This indicates stronger many-body interactions in proximity of the band insulator regime, which we attribute to the presence of unusual magnetic excitations.
قيم البحث
اقرأ أيضاً
The Lieb lattice possesses three bands and with intrinsic spin orbit coupling $lambda$, supports topologically non-trivial band insulating phases. At half filling the lower band is fully filled, while the upper band is empty. The chemical potential l
ies in the flat band (FB) located at the middle of the spectrum, thereby stabilizing a flat band insulator. At this filling, we introduce on-site Hubbard interaction $U$ on all sites. Within a slave rotor mean field theory we show that, in spite of the singular effect of interaction on the FB, the three bands remain stable up to a fairly large critical correlation strength ($U_{crit}$), creating a correlated flat band insulator. Beyond $U_{crit}$, there is a sudden transition to a Mott insulating state, where the FB is destroyed due to complete transfer of spectral weight from the FB to the upper and lower bands. We show that all the correlation driven insulating phases host edge modes with linearly dispersing bands along with a FB passing through the Dirac point, exhibiting that the topological nature of the bulk band structure remains intact in presence of strong correlation. Furthermore, in the limiting case of $U$ introduced only on one sublattice where $lambda=0$, we show that the Lieb lattice can support mixed edge modes containing contributions from both spinons and electrons, in contrast to purely spinon edge modes arising in the topological Mott insulator.
We present an explanation for the puzzling spectral and transport properties of layered cobaltates close to the band-insulator limit, which relies on the key effect of charge ordering. Blocking a significant fraction of the lattice sites deeply modif
ies the electronic structure in a way that is shown to be quantitatively consistent with photoemission experiments. It also makes the system highly sensitive to interactions (especially to intersite ones), hence accounting for the strong correlations effects observed in this regime, such as the high effective mass and quasiparticle scattering rate. These conclusions are supported by a theoretical study of an extended Hubbard model with a realistic band structure on an effective kagom`e lattice.
We present a comparative study of CoO2 layers in the Bi-misfit and NaxCoO2 cobaltates. Co NMR measures the intrinsic susceptibility of the Co layers and is not affected by spurious contributions. At low dopings where room-temperature thermopower (TEP
) is large, Curie-Weiss susceptibilities are observed in both materials. But NMR and muSR experiments find neither charge nor spin order down to low temperatures in Bi-misfit, in contrast to the case of NaxCoO2. This demonstrates that metallicity, charge and magnetic orders are specific of the Na layers in NaxCoO2 whereas strong correlations are generic of the cobaltates physics and could explain the large TEP.
The surface band bending tunes considerably the surface band structures and transport properties in topological insulators. We present a direct measurement of the band bending on the Bi2Se3 by using the bulk sensitive angular-resolved hard x-ray phot
ospectroscopy (HAXPES). We tracked the depth dependence of the energy shift of Bi and Se core states. We estimate that the band bending extends up to about 20 nm into the bulk with an amplitude of 0.23--0.26 eV, consistent with profiles previously deduced from the binding energies of surface states in this material.
A 59Co NMR study of CoO2, the x=0 end member of AxCoO2 (A = Na, Li...) cobaltates, reveals a metallic ground state, though with clear signs of strong electron correlations: low-energy spin fluctuations develop at wave vectors q different from 0 and a
crossover to a Fermi-liquid regime occurs below a characteristic temperature T*~7 K. Despite some uncertainty over the exact cobalt oxidation state n this material, the results show that electronic correlations are revealed as x is reduced below 0.3. The data are consistent with NaxCoO2 being close to the Mott transition in the x -> 0 limit.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
