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We have recorded fluorescence spectra of the atomic rubidium D-lines in the presence of several hundreds of bars buffer gas pressure. With additional saturation broadening a spectral linewidth comparable to the thermal energy of the atoms in the heated gas cell is achieved. An intensity-dependent blue asymmetry of the spectra is observed, which becomes increasingly pronounced when extrapolating to infinitely high light intensity. We interpret our results as evidence for the dressed (coupled atom-light) states to approach thermal equilibrium.
We describe measurements demonstrating laser cooling of an atomic gas by means of collisional redistribution of radiation. The experiment uses rubidium atoms in the presence of several hundred bar of argon buffer gas pressure. Frequent collisions in
Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra-violet) -- IR (infrared) measuremen
We report on the demonstration of Doppler-free polarization spectroscopy of the D2 line of 6Li atoms. Counterintuitively, the presence of an Ar buffer gas, in a certain pressure range, causes a drastic enhancement of the polarization rotation signal.
We report modulation transfer spectroscopy on the D2 transitions in 85Rb and 87Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87Rb F=2 to F
We demonstrate cryogenic buffer-gas cooling of gas-phase methyltrioxorhenium (MTO). This molecule is closely related to chiral organometallic molecules where the parity-violating energy differences between enantiomers may be measurable. The molecules