Direct comparison of optical lattice clocks with an intercontinental baseline of 9 000 km

We have demonstrated a direct frequency comparison between two $^{87}{rm Sr}$ lattice clocks operated in intercontinentally separated laboratories in real time. Two-way satellite time and frequency transfer technique based on the carrier phase was employed for a direct comparison with a baseline of 9 000 km between Japan and Germany. A clock comparison was achieved for 83 640 s resulting in a fractional difference of $(1.1pm1.6) times 10^{-15}$, where the statistical part is the biggest contribution to the uncertainty. This measurement directly confirms the agreement of the two optical clocks on an intercontinental scale.

Carrier-phase Two-Way Satellite Frequency Transfer over a Very Long Baseline

In this paper we report that carrier-phase two-way satellite time and frequency transfer (TWSTFT) was successfully demonstrated over a very long baseline of 9,000 km, established between the National Institute of Information and Communications Technology (NICT) and the Physikalisch-Technische Bundesanstalt (PTB). We verified that the carrier-phase TWSTFT (TWCP) result agreed with those obtained by conventional TWSTFT and GPS carrier-phase (GPSCP) techniques. Moreover, a much improved short-term instability for frequency transfer of $2times10^{-13}$ at 1 s was achieved, which is at the same level as previously confirmed over a shorter baseline within Japan. The precision achieved was so high that the effects of ionospheric delay became significant which are ignored in conventional TWSTFT even over a long link. We compensated for these effects using ionospheric delays computed from regional vertical total electron content maps. The agreement between the TWCP and GPSCP results was improved because of this compensation.

Direct comparison of a Ca+ single ion clock against a Sr optical lattice clock

Optical frequency comparison of the 40Ca+ clock transition u_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition u_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio u_{Ca} / u_{Sr} = 0.957 631 202 358 049 9(2 3). The rapid nature of optical comparison allowed the statistical uncertainty of frequency ratio u_{Ca} / u_{Sr} to reach 1x10-15 in only 1000s and yielded a value consistent with that calculated from separate absolute frequency measurements of u_{Ca} using the International Atomic Time (TAI) link. The total uncertainty of the frequency ratio using optical comparison (free from microwave link uncertainties) is smaller than that obtained using absolute frequency measurement, demonstrating the advantage of optical frequency evaluation. We report the absolute frequency of ^{40}Ca+ with a systematic uncertainty 14 times smaller than our previous measurement [1].

Stability Transfer between Two Clock Lasers Operating at Different Wavelengths for Absolute Frequency Measurement of Clock Transition in 87Sr

We demonstrated transferring the stability of one highly stable clock laser operating at 729 nm to another less stable laser operating at 698 nm. The two different wavelengths were bridged using an optical frequency comb. The improved stability of the clock laser at 698 nm enabled us to evaluate the systematic frequency shifts of the Sr optical lattice clock with shorter averaging time. We determined the absolute frequency of the clock transition 1S0 - 3P0 in 87Sr to be 429 228 004 229 873.9 (1.4) Hz referenced to the SI second on the geoid via International Atomic Time (TAI).

All-optical link for direct comparison of distant optical clocks

We developed an all-optical link system for making remote comparisons of two distant ultra-stable optical clocks. An optical carrier transfer system based on a fiber interferometer was employed to compensate the phase noise accumulated during the propagation through a fiber link. Transfer stabilities of $2times10^{-15}$ at 1 second and $4times10^{-18}$ at 1000 seconds were achieved in a 90-km link. An active polarization control system was additionally introduced to maintain the transmitted light in an adequate polarization, and consequently, a stable and reliable comparison was accomplished. The instabilities of the all-optical link system, including those of the erbium doped fiber amplifiers (EDFAs) which are free from phase-noise compensation, were below $2times10^{-15}$ at 1 second and $7times10^{-17}$ at 1000 seconds. The system was available for the direct comparison of two distant $^{87}$Sr lattice clocks via an urban fiber link of 60 km. This technique will be essential for the measuring the reproducibility of optical frequency standards.

Direct Comparison of Distant Optical Lattice Clocks at the $10^{-16}$ Uncertainty

Fiber-based remote comparison of $^{87}$Sr lattice clocks in 24 km distant laboratories is demonstrated. The instability of the comparison reaches $5times10^{-16}$ over an averaging time of 1000 s, which is two orders of magnitude shorter than that of conventional satellite links and is limited by the instabilities of the optical clocks. By correcting the systematic shifts that are predominated by the differential gravitational redshift, the residual fractional difference is found to be $(1.0pm7.3)times10^{-16}$, confirming the coincidence between the two clocks. The accurate and speedy comparison of distant optical clocks paves the way for a future optical redefinition of the second.

Buffer gas induced collision shift for the $^{88}$Sr $bf{^1S_0-^3P_1}$ clock transition

Precision saturation spectroscopy of the $^{88}{rm Sr} ^1S_0-^3P_1$ is performed in a vapor cell filled with various rare gas including He, Ne, Ar, and Xe. By continuously calibrating the absolute frequency of the probe laser, buffer gas induced collision shifts of $sim $kHz are detected with gas pressure of 1-20 mTorr. Helium gave the largest fractional shift of $1.6 times 10^{-9} {rm Torr}^{-1}$. Comparing with a simple impact calculation and a Doppler-limited experiment of Holtgrave and Wolf [Phys. Rev. A {bf 72}, 012711 (2005)], our results show larger broadening and smaller shifting coefficient, indicating effective atomic loss due to velocity changing collisions. The applicability of the result to the $^1S_0-^3P_0$ optical lattice clock transition is also discussed.