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Modern x-ray light sources promise access to structure and dynamics of matter in largely unexplored spectral regions. However, the desired information is encoded in the light intensity and phase, whereas detectors register only the intensity. This ph ase problem is ubiquitous in crystallography and imaging, and impedes the exploration of quantum effects at x-ray energies. Here, we demonstrate phase-sensitive measurements characterizing the quantum state of a nuclear two-level system at hard x-ray energies. The nuclei are initially prepared in a superposition state. Subsequently, the relative phase of this superposition is interferometrically reconstructed from the emitted x-rays. Our results form a first step towards x-ray quantum state tomography, and provide new avenues for structure determination and precision metrology via x-ray Fano interference.
Group velocity control is demonstrated for x-ray photons of 14.4 keV energy via a direct measurement of the temporal delay imposed on spectrally narrow x-ray pulses. Sub-luminal light propagation is achieved by inducing a steep positive linear disper sion in the optical response of ${}^{57}$Fe Mossbauer nuclei embedded in a thin film planar x-ray cavity. The direct detection of the temporal pulse delay is enabled by generating frequency-tunable spectrally narrow x-ray pulses from broadband pulsed synchrotron radiation. Our theoretical model is in good agreement with the experimental data.
109 - L. Zhang , J. Evers 2013
A setup to frequency-convert an arbitrary image encoded in the spatial profile of a probe field onto a signal field using four-wave mixing in a thermal atom vapor is proposed. The atomic motion is exploited to cancel diffraction of both signal and pr obe fields simultaneously. We show that an incoherent probe field can be used to enhance the transverse momentum bandwidth which can be propagated without diffraction, such that smaller structures with higher spatial resolution can be transmitted. It furthermore compensate linear absorption with non-linear gain, to improve the four-wave mixing performance since the propagation dynamics of the various field intensities is favorably modified.
The control of light-matter interaction at the quantum level usually requires coherent laser fields. But already an exchange of virtual photons with the electromagnetic vacuum field alone can lead to quantum coherences, which subsequently suppress sp ontaneous emission. We demonstrate such spontaneously generated coherences (SGC) in a large ensemble of nuclei operating in the x-ray regime, resonantly coupled to a common cavity environment. The observed SGC originates from two fundamentally different mechanisms related to cooperative emission and magnetically controlled anisotropy of the cavity vacuum. This approach opens new perspectives for quantum control, quantum state engineering and simulation of quantum many-body physics in an essentially decoherence-free setting.
Applications of negative index materials (NIM) presently are severely limited by absorption. Next to improvements of metamaterial designs, it has been suggested that dense gases of atoms could form a NIM with negligible losses. In such gases, the low absorption is facilitated by quantum interference. Here, we show that additional gain mechanisms can be used to tune and effectively remove absorption in a dense gas NIM. In our setup, the atoms are coherently prepared by control laser fields, and further driven by a weak incoherent pump field to induce gain. We employ nonlinear optical Bloch equations to analyze the optical response. Metastable Neon is identified as a suitable experimental candidate at infrared frequencies to implement a lossless active negative index material.
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