The advent of accelerator-driven free-electron lasers (FEL) has opened new avenues for high-resolution structure determination via diffraction methods that go far beyond conventional x-ray crystallography methods. These techniques rely on coherent sc
attering processes that require the maintenance of first-order coherence of the radiation field throughout the imaging procedure. Here we show that higher-order degrees of coherence, displayed in the intensity correlations of incoherently scattered x-rays from an FEL, can be used to image two-dimensional objects with a spatial resolution close to or even below the Abbe limit. This constitutes a new approach towards structure determination based on incoherent processes, including Compton scattering, fluorescence emission or wavefront distortions, generally considered detrimental for imaging applications. Our method is an extension of the landmark intensity correlation measurements of Hanbury Brown and Twiss to higher than second-order paving the way towards determination of structure and dynamics of matter in regimes where coherent imaging methods have intrinsic limitations.
Superradiance is one of the outstanding problems in quantum optics since Dicke introduced the concept of enhanced directional spontaneous emission by an ensemble of identical two-level atoms. The effect is based on correlated collective Dicke states
which turn out to be highly entangled. Here we show that enhanced directional emission of spontaneous radiation can be produced also with statistically independent incoherent sources via the measurement of higher order correlation functions of the emitted radiation. Our analysis is applicable to a wide variety of quantum systems like trapped atoms, ions, quantum dots or NV-centers, and is also valid for statistically independent incoherent classical emitters. This is experimentally confirmed with up to eight independent thermal light sources.
We present a mathematical proof of the algorithm allowing to generate all - symmetric and non-symmetric - total angular momentum eigenstates in remote matter qubits by projective measurements, proposed in Maser et al. [Phys. Rev. A 79, 033833 (2009)]
. By deriving a recursion formula for the algorithm we show that the generated states are equal to the total angular momentum eigenstates obtained via the usual quantum mechanical coupling of angular momenta. In this way we demonstrate that the algorithm is able to simulate the coupling of N spin-1/2 systems, and to implement the required Clebsch-Gordan coefficients, even though the particles never directly interact with each other.
We propose a method for the generation of a large variety of entangled states, encoded in the polarization degrees of freedom of N photons, within the same experimental setup. Starting with uncorrelated photons, emitted from N arbitrary single photon
sources, and using linear optical tools only, we demonstrate the creation of all symmetric states, e.g., GHZ- and W-states, as well as all symmetric and non-symmetric total angular momentum eigenstates of the N qubit compound.
The different behaviour of first order interferences and second order correlations are investigated for the case of two coherently excited atoms. For intensity measurements this problem is equivalent to Youngs double slit experiment and was investiga
ted in an experiment by Eichmann et al. [Phys. Rev. Lett. 70, 2359 (1993)] and later analyzed in detail by Itano et al. [Phys. Rev. A 57, 4176 (1998)]. Our results show that in cases where the intensity interferences disappear the intensity-intensity correlations can display an interference pattern with a visibility of up to 100%. The contrast depends on the polarization selected for the detection and is independent of the strength of the driving field. The nonclassical nature of the calculated intensity-intensity correlations is also discussed.
The emission characteristics in the fluorescence of two laser-driven dipole-dipole-interacting three level atoms is investigated. When the light from both atoms is detected separately a correlation of the emission processes is observed in dependence
of the dipole-dipole interaction. This opens the possibility to investigate the dipole-dipole interaction through the emission behavior. We present Monte-Carlo simulations which are in good agreement with the analytic solutions.
We demonstrate the existence of new nonclassical correlations in the radiation of two atoms, which are coherently driven by a continuous laser source. The photon-photon-correlations of the fluorescence light show a spatial interferene pattern not pre
sent in a classical treatment. A feature of the new phenomenon is, that bunched and antibunched light is emitted in different spatial directions. The calculations are performed analytically. It is pointed out, that the correlations are induced by state reduction due to the measurement process when the detection of the photons does not distinguish between the atoms. It is interesting to note, that the phenomena show up even without any interatomic interaction.
The absolute frequency of the In$^{+}$ $5s^{2 1}S_{0}$ - $5s5p^{3}P_{0}$ clock transition at 237 nm was measured with an accuracy of 1.8 parts in $10^{13}$. Using a phase-coherent frequency chain, we compared the $^{1}S_{0}$ - $^{3}P_{0}$ transition
with a methane-stabilized He-Ne laser at 3.39 $mu$m which was calibrated against an atomic cesium fountain clock. A frequency gap of 37 THz at the fourth harmonic of the He-Ne standard was bridged by a frequency comb generated by a mode-locked femtosecond laser. The frequency of the In$^{+}$ clock transition was found to be $1 267 402 452 899.92 (0.23)$ kHz, the accuracy being limited by the uncertainty of the He-Ne laser reference. This represents an improvement in accuracy of more than 2 orders of magnitude on previous measurements of the line and now stands as the most accurate measurement of an optical transition in a single ion.
We consider pump-probe spectroscopy of a single ion with a highly metastable (probe) clock transition which is monitored by using the quantum jump technique. For a weak clock laser we obtain the well known Autler-Townes splitting. For stronger powers
of the clock laser we demonstrate the transition to a new regime. The two regimes are distinguished by the transition of two complex eigenvalues to purely imaginary ones which can be very different in magnitude. The transition is controlled by the power of the clock laser. For pump on resonance we present simple analytical expressions for various linewidths and line positions.
