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The KADoNiS (Karlsruhe Astrophysical Database of Nucleosynthesis in Stars) project is an astrophysical online database for cross sections relevant for nucleosynthesis in the $s$ process and the $gamma$ process. The $s$-process database (www.kadonis.o rg) was started in 2005 and is presently facing its 4th update (KADoNiS v1.0). The $gamma$-process database (KADoNiS-p, www.kadonis.org/pprocess) was recently revised and re-launched in March 2013. Both databases are compilations for experimental cross sections with relevance to heavy ion nucleosynthesis. For the $s$ process recommended Maxwellian averaged cross sections for $kT$= 5-100~keV are given for more than 360 isotopes between $^{1}$H and $^{210}$Bi. For the $gamma$-process database all available experimental data from $(p,gamma), (p,n), (p,alpha), (alpha,gamma), (alpha,n)$, and $(alpha,p)$ reactions between $^{70}$Ge and $^{209}$Bi in or close to the respective Gamow window were collected and can be compared to theoretical predictions. The aim of both databases is a quick and user-friendly access to the available data in the astrophysically relevant energy regions.
Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E_p=2.75 MeV to 9 MeV, close to the upper end of the respective Gamow window of the gamma process. We have det ermined cross sections for 102Pd(p,gamma)103Ag, 104Pd(p,gamma)105Ag, and 105Pd(p,n)105Ag, as well as partial cross sections of 104Pd(p,n)104Ag^g, 105Pd(p,gamma)106Ag^m, 106Pd(p,n)106Ag^m, and 110Pd(p,n)110Ag^m with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.
We have investigated the (n,gamma) cross sections of p-process isotopes with the activation technique. The measurements were carried out at the Karlsruhe Van de Graaff accelerator using the 7Li(p,n)7Be source for simulating a Maxwellian neutron distr ibution of kT = 25 keV. Stellar cross section measurements are reported for the light p-process isotopes 102Pd, 120Te, 130,132Ba, and 156Dy. In a following paper the cross sections of 168Yb, 180W, 184Os, 190Pt, and 196Hg will be discussed. The data are extrapolated to p-process energies by including information from evaluated nuclear data libraries. The results are compared to standard Hauser-Feshbach models frequently used in astrophysics.
The discovery of naturally occurring long-lived isomeric states (t_1/2 > 10^8 yr) in the neutron-deficient isotopes 211,213,217,218Th [A. Marinov et al., Phys. Rev. C 76, 021303(R) (2007)] was reexamined using accelerator mass spectrometry (AMS). Bec ause AMS does not suffer from molecular isobaric background in the detection system, it is an extremely sensitive technique. Despite our up to two orders of magnitude higher sensitivity we cannot confirm the discoveries of neutron-deficient thorium isotopes and provide upper limits for their abundances.
An accurate knowledge of the neutron capture cross sections of 62,63Ni is crucial since both isotopes take key positions which affect the whole reaction flow in the weak s process up to A=90. No experimental value for the 63Ni(n,gamma) cross section exists so far, and until recently the experimental values for 62Ni(n,gamma) at stellar temperatures (kT=30 keV) ranged between 12 and 37 mb. This latter discrepancy could now be solved by two activations with following AMS using the GAMS setup at the Munich tandem accelerator which are also in perfect agreement with a recent time-of-flight measurement. The resulting (preliminary) Maxwellian cross section at kT=30 keV was determined to be <sigma>30keV = 23.4 +/- 4.6 mb. Additionally, we have measured the 64Ni(gamma,n)63Ni cross section close to threshold. Photoactivations at 13.5 MeV, 11.4 MeV and 10.3 MeV were carried out with the ELBE accelerator at Forschungszentrum Dresden-Rossendorf. A first AMS measurement of the sample activated at 13.5 MeV revealed a cross section smaller by more than a factor of 2 compared to NON-SMOKER predictions.
The stellar (n,gamma) cross section of 40Ca at kT=25 keV has been measured with a combination of the activation technique and accelerator mass spectrometry (AMS). This combination is required when direct off-line counting of the produced activity is compromised by the long half-life and/or missing gamma-ray transitions. The neutron activations were performed at the Karlsruhe Van de Graaff accelerator using the quasistellar neutron spectrum of kT=25 keV produced by the 7Li(p,n)7Be reaction. The subsequent AMS measurements were carried out at the Vienna Environmental Research Accelerator (VERA) with a 3 MV tandem accelerator. The doubly magic 40Ca is a bottle-neck isotope in incomplete silicon burning, and its neutron capture cross section determines the amount of leakage, thus impacting on the eventual production of iron group elements. Because of its high abundance, 40Ca can also play a secondary role as neutron poison for the s-process. Previous determinations of this value at stellar energies were based on time-of-flight measurements. Our method uses an independent approach, and yields for the Maxwellian-averaged cross section at kT=30 keV a value of <sigma>30 keV= 5.73+/-0.34 mb.
The $^{92}$Mo($alpha,n$)$^{95}$Ru, $^{94}$Mo($alpha,n$)$^{97}$Ru, and $^{112}$Sn($alpha,gamma$)$^{116}$Te cross sections were measured at the upper end of the $p$-process Gamow window between 8.2 MeV and 11.1 MeV. Our results are slightly lower than global Hauser-Feshbach calculations from the code NON-SMOKER, but still within the uncertainty of the prediction. The $^{112}$Sn($alpha,gamma$)$^{116}$Te cross section agrees well with a recently measured thick-target cross section in the same energy range. For the $^{92,94}$Mo($alpha,n$) reactions the present data close to the reaction thresholds could eliminate previous uncertainties within a factor of 20, and we can present now useful comparisons to statistical model calculations with different optical potentials.
Since April 2005 a regularly updated stellar neutron cross section compilation is available online at http://nuclear-astrophysics.fzk.de/kadonis. This online-database is called the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project and is based on the previous Bao et al. compilation from the year 2000. The present version textsc{KADoNiS} v0.2 (January 2007) includes recommended cross sections for 280 isotopes between $^{1}$H and $^{210}$Po and 75 semi-empirical estimates for isotopes without experimental information. Concerning stellar $(n,gamma)$ cross sections of the 32 stable, proton-rich isotopes produced by the $p$ process experimental information is only available for 20 isotopes, but 9 of them have rather large uncertainties of $geq$9%. The first part of a systematic study of stellar $(n,gamma)$ cross sections of the $p$-process isotopes $^{74}$Se, $^{84}$Sr, $^{102}$Pd, $^{120}$Te, $^{130}$Ba, $^{132}$Ba, $^{156}$Dy, and $^{174}$Hf is presented. In another application textsc{KADoNiS} v0.2 was used for an modification of a reaction library of Basel university. With this modified library $p$-process network calculations were carried out and compared to previous results.
75 - I. Dillmann , R. Plag , M. Heil 2008
The Karlsruhe Astrophysical Database of Nucleosynthesis in Stars (KADoNiS) project is an online database for experimental cross sections relevant to the $s$ process and $p$ process. It is available under http://nuclear-astrophysics.fzk.de/kadonis and consists of two parts. Part 1 is an updated sequel to the well-known Bao et al. compilations from 1987 and 2000, which is online since April 2005. An extension of this $s$-process database to $(n,p)$ and $(n,alpha)$ cross sections at $kT$= 30 keV, as in the first version of the Bao compilation, is planned. The second part of KADoNiS is a $p$-process library, which includes all available experimental data from $(p,gamma)$, $(p,n)$, $(alpha,gamma)$, $(alpha,n)$, $(alpha,alpha)$, $(n,alpha)$ and $(gamma,n)$ reactions in or close to the respective Gamow window. Despite the great number of reactions required for a $p$-process reaction network, experimental data is still scarce and up to now restricted to stable targets. Given here is a short overview about the present status of the KADoNiS database.
We have performed $p$-process simulations with the most recent stellar $(n,gamma)$ cross sections from the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project (version v0.2, http://nuclear-astrophysics.fzk.de/kadonis). The simulation s were carried out with a parametrized supernova type II shock front model (``$gamma$ process) of a 25 solar mass star and compared to recently published results. A decrease in the normalized overproduction factor could be attributed to lower cross sections of a significant fraction of seed nuclei located in the Bi and Pb region around the $N$=126 shell closure.
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