We demonstrate a simple scheme for high-resolution imaging of nanoplasmonic structures that basically removes most of the resolution limiting allowed light usually transmitted to the far field. This is achieved by implementing a Fourier lens in a nea
r-field scanning optical microscope (NSOM) operating in the leakage-radiation microscopy (LRM) mode. The method consists of reconstructing optical images solely from the plasmonic `forbidden light collected in the Fourier space. It is demonstrated by using a point-like nanodiamond-based tip that illuminates a thin gold film patterned with a sub-wavelength annular slit. The reconstructed image of the slit shows a spatial resolution enhanced by a factor $simeq 4$ compared to NSOM images acquired directly in the real space.
We develop a semi-analytical method for analyzing surface plasmon interferometry using near-field scanning optical sources. We compare our approach to Young double hole interferometry experiments using scanning tunneling microscope (STM) discussed in
the literature and realize experiments with an aperture near-field scanning optical microscope (NSOM) source positioned near a ring like aperture slit milled in a thick gold film. In both cases the agreement between experiments and model is very good. We emphasize the role of dipole orientations and discuss the role of magnetic versus electric dipole contributions to the imaging process as well as the directionality of the effective dipoles associated with the various optical and plasmonic sources.
We show that, contrary to the common wisdom, surface plasmon poles are not involved in the imaging process in leakage radiation microscopy. Identifying the leakage radiation modes directly from a transverse magnetic potential leads us to reconsider t
he surface plasmon field and unfold the non-plasmonic contribution to the image formation. While both contributions interfere in the imaging process, our analysis reveals that the reassessed plasmonic field embodies a pole mathematically similar to the usual surface plasmon pole. This removes a long-standing ambiguity associated with plasmonic signals in leakage radiation microscopy.
Light interacts differently with left and right handed three dimensional chiral objects, like helices, and this leads to the phenomenon known as optical activity. Here, by applying a polarization tomography, we show experimentally, for the first time
in the visible domain, that chirality has a different optical manifestation for twisted planar nanostructured metallic objects acting as isolated chiral metaobjects. Our analysis demonstrate how surface plasmons, which are lossy bidimensional electromagnetic waves propagating on top of the structure, can delocalize light information in the just precise way for giving rise to this subtle effect.
We introduce a point-like scanning single-photon source that operates at room temperature and offers an exceptional photostability (no blinking, no bleaching). This is obtained by grafting in a controlled way a diamond nanocrystal (size around 20 nm)
with single nitrogen-vacancy color-center occupancy at the apex of an optical probe. As an application, we image metallic nanostructures in the near-field, thereby achieving a near-field scanning single-photon microscopy working at room temperature on the long term. Our work may be of importance to various emerging fields of nanoscience where an accurate positioning of a quantum emitter is required such as for example quantum plasmonics.
