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187 - A. Singer , M. Marsh , S. Dietze 2014
Here we report on the dynamics of the structural order parameter in a chromium film using synchrotron radiation in response to photo-induced ultra-fast excitations. Following transient optical excitations the effective lattice temperature of the film rises close to the N{e}el temperature and the charge density wave (CDW) amplitude is reduced. Although we expect the electronic charge ordering to vanish shortly after the excitation we observe that the CDW is never completely disrupted, which is revealed by its unmodified period at elevated temperatures. We attribute the persistence of the CDW to the long-lived periodic lattice displacement in chromium. The long-term evolution shows that the CDW revives to its initial strength within 1 ns, which appears to behave in accordance with the temperature dependence in equilibrium. This study highlights the fundamental role of the lattice distortion in charge ordered systems and its impact on the re-condensation dynamics of the charge ordered state in strongly correlated materials.
A general theoretical approach based on the results of statistical optics is used for the analysis of the transverse coherence properties of 3-rd generation synchrotron sources and x-ray free-electron lasers (XFEL). Correlation properties of the wave fields are calculated at different distances from an equivalent Gaussian Schell-model source. This model is used to describe coherence properties of the five meter undulator source at the synchrotron storage ring PETRA III. In the case of XFEL sources the decomposition of the statistical fields into a sum of independently propagating transverse modes is used for the analysis of the coherence properties of these new sources. A detailed calculation is performed for the parameters of the SASE1 undulator at the European XFEL. It is demonstrated that only a few modes contribute significantly to the total radiation field of that source.
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