We expand the concept of frustration in Mott insulators and quantum spin liquids to metals with flat bands. We show that when inter-orbital hopping $t_2$ dominates over intra-orbital hopping $t_1$, in a multiband system with strong spin-orbit couplin
g $lambda$, electronic states with a narrow bandwidth $Wsim t_2^2/lambda$ are formed compared to a bandwidth of order $t_1$ for intra-orbital hopping. We demonstrate the evolution of the electronic structure, Berry phase distributions for time-reversal and inversion breaking cases, and their imprint on the optical absorption, in a tight binding model of $d$-orbital hopping on a honeycomb lattice. Going beyond quantum Hall effect and twisted bilayer graphene, we provide an alternative mechanism and a richer materials platform for achieving flat bands poised at the brink of instabilities toward novel correlated and fractionalized metallic phases.
Quadrupole topological phases, exhibiting protected boundary states that are themselves topological insulators of lower dimensions, have recently been of great interest. Extensions of these ideas from current tight binding models to continuum theorie
s for realistic materials require the identification of quantized invariants describing the bulk quadrupole order. Here we identify the analog of quadrupole order in Maxwells equations for a photonic crystal (PhC) and identify quadrupole topological photonic crystals formed through a band inversion process. Unlike prior studies relying on threaded flux, our quadrupole moment is quantized purely by crystalline symmetries, which we confirm using three independent methods: analysis of symmetry eigenvalues, numerical calculations of the nested Wannier bands, and the expectation value of the quadrupole operator. Furthermore, through the bulk-edge correspondence of Wannier bands, we reveal the boundary manifestations of nontrivial quadrupole phases as quantized polarizations at edges and bound states at corners. Finally, we relate the nontrivial corner states to the emergent phenomena of quantized fractional corner charges and a filling anomaly as first predicted in electronic systems. Our work paves the way to further explore higher-order topological phases in nanophotonic systems and our method of inducing quadrupole phase transitions is also applicable to other wave systems, such as electrons, phonons and polaritons.
Achieving topologically-protected robust transport in optical systems has recently been of great interest. Most topological photonic structures can be understood by solving the eigenvalue problem of Maxwells equations for a static linear system. Here
, we extend topological phases into dynamically driven nonlinear systems and achieve a Floquet Chern insulator of light in nonlinear photonic crystals (PhCs). Specifically, we start by presenting the Floquet eigenvalue problem in driven two-dimensional PhCs and show it is necessarily non-Hermitian. We then define topological invariants associated with Floquet bands using non-Hermitian topological band theory, and show that topological band gaps with non-zero Chern number can be opened by breaking time-reversal symmetry through the driving field. Furthermore, we show that topological phase transitions between Floquet Chern insulators and normal insulators occur at synthetic Weyl points in a three-dimensional parameter space consisting of two momenta and the driving frequency. Finally, we numerically demonstrate the existence of chiral edge states at the interfaces between a Floquet Chern insulator and normal insulators, where the transport is non-reciprocal and uni-directional. Our work paves the way to further exploring topological phases in driven nonlinear optical systems and their optoelectronic applications, and our method of inducing Floquet topological phases is also applicable to other wave systems, such as phonons, excitons, and polaritons.
Weyl semimetals are gapless topological states of matter with broken inversion and/or time reversal symmetry, which can support unconventional responses to externally applied electrical, optical and magnetic fields. Here we report a new photogalvanic
effect in type-II WSMs, MoTe2 and Mo0.9W0.1Te2, which are observed to support a circulating photocurrent when illuminated by circularly polarized light at normal incidence. This effect occurs exclusively in the inversion broken phase, where crucially we find that it is associated with a spatially varying beam profile via a new dispersive contribution to the circular photogalvanic effect (s-CPGE). The response functions derived for s-CPGE reveal the microscopic mechanism of this photocurrent, which are controlled by terms that are allowed in the absence of inversion symmetry, along with asymmetric carrier excitation and relaxation. By evaluating this response for a minimal model of a Weyl semimetal, we obtain the frequency dependent scaling behavior of this form of photocurrent. These results demonstrate opportunities for controlling photoresponse by patterning optical fields to store, manipulate and transmit information over a wide spectral range.
