Optical whispering gallery mode (WGM) resonators have been very attracting platforms for versatile Kerr frequency comb generations. We report a systematic study on the material dispersion of various optical materials that are capable of supporting qu
ality factors above $10^9$. Using an analytical approximation of WGM resonant frequencies in disk resonators, we investigate the effect of the geometry and transverse mode order on the total group-velocity dispersion ($GVD$). We demonstrate that the major radii and the radial mode indices play an important role in tailoring the $GVD$ of WGM resonators. In particular, our study shows that in WGM disk-resonators, the polar families of modes have very similar $GVD$, while the radial families of modes feature dispersion values that can differ by up to several orders of magnitude. The effect of these giant dispersion shifts are experimentally evidenced in Kerr comb generation with magnesium fluoride. From a more general perspective, this critical feature enables to push the zero-dispersion wavelength of fluorite crystals towards the mid-infrared (mid-IR) range, thereby allowing for efficient Kerr comb generation in that spectral range. We show that barium fluoride is the most interesting crystal in this regard, due to its zero dispersion wavelength ($ZDW$) at $1.93 rm{mu m}$ and an optimal dispersion profile in the mid-IR regime. We expect our results to facilitate the design of different platforms for Kerr frequency comb generations in both telecommunication and mid-IR spectral ranges.
In this article, we use quantum Langevin equations to provide a theoretical understanding of the non-classical behavior of Kerr optical frequency combs when pumped below and above threshold. In the configuration where the system is under threshold, t
he pump field is the unique oscillating mode inside the resonator, and triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various sidemodes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double peaked depending on the parameters of the system. We also calculate as well the overall spontaneous noise power per sidemode, and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatio-temporal patterns, the side-modes that are symmetrical relatively to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light. We also explicitly determine the phase quadratures leading to photon entanglement, and analytically calculate their quantum noise spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths, below and above threshold.
We theoretically investigate the phase-locking phenomena between the spectral components of Kerr optical frequency combs in the dynamical regime of Turing patterns. We show that these Turing patterns display a particularly strong and robust phase-loc
king, originating from a cascade of phase-locked triplets which asymptotically lead to a global phase-locking between the modes. The local and global phase-locking relationship defining the shape of the optical pulses are analytically determined. Our analysis also shows that solitons display a much weaker phase-locking which can be destroyed more easily than in the Turing pattern regime. Our results indicate that Turing patterns are generally the most suitable for applications requiring the highest stability. Experimental generation of such combs is also discussed in detail, in excellent agreement with the numerical simulations.
We investigate the various routes to spatiotemporal chaos in Kerr optical frequency combs obtained through pumping an ultra-high quality whispering-gallery mode resonator with a continuous-wave laser. The Lugiato-Lefever model is used to build bifurc
ation diagrams with regards to the parameters that are externally controllable, namely, the frequency and the power of the pumping laser. We show that the spatiotemporal chaos emerging from Turing patterns and solitons display distinctive dynamical features. Experimental spectra of chaotic Kerr combs are also presented for both cases, in excellent agreement with theoretical spectra.
