The $gamma$-process in core-collapse and/or type Ia supernova explosions is thought to explain the origin of the majority of the so-called $p$ nuclei (the 35 proton-rich isotopes between Se and Hg). Reaction rates for $gamma$-process reaction network
studies have to be predicted using Hauser-Feshbach statistical model calculations. Recent investigations have shown problems in the prediction of $alpha$-widths at astrophysical energies which are an essential input for the statistical model. It has an impact on the reliability of abundance predictions in the upper mass range of the $p$ nuclei. With the measurement of the $^{164,166}$Er($alpha$,n)$^{167,169}$Yb reaction cross sections at energies close to the astrophysically relevant energy range we tested the recently suggested low energy modification of the $alpha$+nucleus optical potential in a mass region where $gamma$-process calculations exhibit an underproduction of the $p$ nuclei. Using the same optical potential for the $alpha$-width which was derived from combined $^{162}$Er($alpha$,n) and $^{162}$Er($alpha$,$gamma$) measurement makes it plausible that a low-energy modification of the optical $alpha$+nucleus potential is needed.
The knowledge of the production of extinct radioactivities like 92Nb and 146Sm by photodisintegration processes in ccSN and SNIa models is essential for interpreting abundances in meteoritic material and for Galactic Chemical Evolution (GCE). The 92M
o/92Nb and 146Sm/144Sm ratios provide constraints for GCE and production sites. We present results for SNIa with emphasis on nuclear uncertainties.
The bulk of p isotopes is created in the gamma processes mainly by sequences of photodisintegrations and beta decays in explosive conditions in Type Ia supernovae (SNIa) or in core collapse supernovae (ccSN). The contribution of different stellar sou
rces to the observed distribution of p-nuclei in the Solar System is still under debate. We explore single degenerate Type Ia supernovae in the framework of two-dimensional SNIa delayed-detonation explosion models. Travaglio et al. (2011, TRV11) discussed the sensitivity of p-nuclei production to different SNIa models, i.e. delayed detonations of different strength, deflagrations, and the dependence on selected s-process seed distributions. Here we present a detailed study of p-process nucleosynthesis occuring in SNIa with s-process seeds at different metallicities. Based on the delayed-detonation model DDT-a of TRV11, we analyze the dependence of p-nucleosynthesis on the s-seed distribution obtained from different strengths of the 13C-pocket. Using a Galactic chemical evolution code (see Travaglio et al. 2004) we study the contribution of SNIa to the solar stable p-nuclei. We find that explosions of Chandrasekhar-mass single degenerate systems produce a large amount of p-nuclei in our Galaxy, both in the range of light (A < 120) and heavy p-nuclei, at almost flat average production factors (within a factor of about 3). We discussed in details p-isotopes such as 94Mo with a behavior diverging from the average, which we attribute to uncertainties in the nuclear data or in SNIa modelling.
The nucleosynthesis of proton-rich isotopes is calculated for multi-dimensional Chandrasekhar-mass models of Type Ia supernovae with different metallicities. The predicted abundances of the short-lived radioactive isotopes 92Nb, 97Tc, 98Tc and 146Sm
are given in this framework. The abundance seeds are obtained by calculating s-process nucleosynthesis in the material accreted onto a carbon-oxygen white dwarf from a binary companion. A fine grid of s-seeds at different metallicities and 13C-pocket efficiencies is considered. A galactic chemical evolution model is used to predict the contribution of SNIa to the solar system p-nuclei composition measured in meteorites. Nuclear physics uncertainties are critical to determine the role of SNeIa in the production of 92Nb and 146Sm. We find that, if standard Chandrasekhar-mass SNeIa are at least 50% of all SNIa, they are strong candidates for reproducing the radiogenic p-process signature observed in meteorites.
A systematic study of the radiative proton capture reaction for all stable nickel isotopes is presented. The results were obtained using 2.0 - 6.0 MeV protons from the 11 MV tandem Van de Graaff accelerator at the University of Notre Dame. The gamma-
rays were detected by the NSCL SuN detector utilising the gamma-summing technique. The results are compared to a compilation of earlier measurements and discrepancies between the previous data are resolved. The experimental results are also compared to the theoretical predictions obtained using the NON-SMOKER and SMARAGD codes. Based on these comparisons an improved set of astrophysical reaction rates is proposed for the (p,gamma) reactions on the stable nickel isotopes as well as for the 56Ni(p,gamma)57Cu reaction.
Modern models of s-process nucleosynthesis in stars require stellar reaction rates with high precision. Most of the neutron capture cross sections in the s-process have been measured and for an increasing number of reactions the required precision is
achieved. This does not necessarily mean, however, that the stellar rates are constrained equally well because only capture on the ground state of a target is measured in the laboratory. Captures on excited states can considerably contribute to stellar rates already at typical s-process temperatures. We show that the ground state contribution X to a stellar rate is the relevant measure to identify reactions which are or could be well constrained by experiments and apply it to (n,gamma) reactions in the s-process. It is further shown that the maximally possible reduction in uncertainty of a rate through determination of the g.s. cross section is directly given by X. An error analysis of X is presented and it is found that X is a robust measure with overall small uncertainties. Several specific examples (neutron capture on 79Se, 95Zr, 121Sn, 187Os, and 193Pt) are discussed in detail. The ground state contributions for a set of 411 neutron capture reactions around the s-process path are presented in a table. This allows to identify reactions which may be better constrained by experiments and such which cannot be constrained by only measuring ground state cross sections (and thus require supplementary studies). General trends and implications are discussed.
It is shown that a Coulomb suppression of the stellar enhancement factor occurs in many endothermic reactions at and far from stability. Contrary to common assumptions, reaction measurements for astrophysics with minimal impact of stellar enhancement
should be preferably performed for those reactions instead of their reverses, despite of their negative reaction Q-value. As a demonstration, the cross section of the astrophysically relevant 85Rb(p,n)85Sr reaction has been measured by activation between 2.16<=E_{c.m.}<= 3.96 MeV and the astrophysical reaction rates at p-process temperatures for (p,n) as well as (n,p) are directly inferred from the data. Additionally, our results confirm a previously derived modification of a global optical proton potential. The presented arguments are also relevant for other alpha- and proton-induced reactions in the p-, rp-, and nu-p-processes.
Primordial molecules were formed during the Dark Ages, i.e. the time between recombination and reionization in the early Universe. The purpose of this article is to analyze the formation of primordial molecules based on heavy elements during the Dark
Ages, with elemental abundances taken from different nucleosynthesis models. We present calculations of the full non-linear equation set governing the primordial chemistry. We consider the evolution of 45 chemical species and use an implicit multistep method of variable order of precision with an adaptive stepsize control. We find that the most abundant Dark Ages molecules based on heavy elements are CH and OH. Non-standard nucleosynthesis can lead to higher heavy element abundances while still satisfying the observed primordial light abundances. In that case, we show that the abundances of molecular species based on C, N, O and F can be enhanced by two orders of magnitude compared to the standard case, leading to a CH relative abundance higher than that of HD+ or H2D+.
We have performed $p$-process simulations with the most recent stellar $(n,gamma)$ cross sections from the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project (version v0.2, http://nuclear-astrophysics.fzk.de/kadonis). The simulation
s were carried out with a parametrized supernova type II shock front model (``$gamma$ process) of a 25 solar mass star and compared to recently published results. A decrease in the normalized overproduction factor could be attributed to lower cross sections of a significant fraction of seed nuclei located in the Bi and Pb region around the $N$=126 shell closure.
The first part of the paper discusses nuclear properties relevant to predict compound reactions. The second part addresses direct reactions with special emphasis on direct neutron capture.
