Bond disorder and breakdown of ballistic heat transport in the spin-1/2 antiferromagnetic Heisenberg chain as seen in Ca-doped SrCuO2

We study the impact of a weak bond disorder on the spinon heat transport in the S=1/2 antiferromagnetic (AFM) Heisenberg chain material Sr_{1-x}Ca_xCuO_2. We observe a drastic suppression in the magnetic heat conductivity kappa_mag even at tiny disorder levels (i.e., Ca-doping levels), in stark contrast to previous findings for kappa_mag of S=1/2 two-dimensional square lattice and two-leg spin-ladder systems, where a similar bond disorder has no effect on kappa_mag. Hence, our results underpin the exceptional role of integrability of the S=1/2 AFM Heisenberg chain model and suggest that the bond disorder effectively destroys the ballistic nature of its heat transport. We further show that the suppression of kappa_mag is captured by an effective spinon-impurity scattering length, which exhibits the same doping dependence as the long-distance exponential decay length of the spin-spin correlation as determined by density-matrix renormalization group calculations.

Ballistic heat transport of quantum spin excitations as seen in SrCuO2

Fundamental conservation laws predict ballistic, i.e., dissipationless transport behaviour in one-dimensional quantum magnets. Experimental evidence, however, for such anomalous transport has been lacking ever since. Here we provide experimental evidence for ballistic heat transport in a S=1/2 Heisenberg chain. In particular, we investigate high purity samples of the chain cuprate SrCuO2 and observe a huge magnetic heat conductivity $kappa_{mag}$. An extremely large spinon mean free path of more than a micrometer demonstrates that $kappa_{mag}$ is only limited by extrinsic scattering processes which is a clear signature of ballistic transport in the underlying spin model.