The blinking dynamics of colloidal core-shell CdSe/CdS dot-in-rods is studied in detail at the single particle level. Analyzing the autocorrelation function of the fluorescence intensity, we demonstrate that these nanoemitters are characterized by a
short value of the mean duration of bright periods (ten to a few hundreds of microseconds). The comparison of the results obtained for samples with different geometries shows that not only the shell thickness is crucial but also the shape of the dot- in-rods. Increasing the shell aspect ratio results in shorter bright periods suggesting that surface traps impact the stability of the fluorescence intensity.
Although it is widely accepted that classical information cannot travel faster than the speed of light in vacuum, the behavior of quantum correlations and quantum information propagating through actively-pumped fast-light media has not been studied i
n detail. To investigate this behavior, we send one half of an entangled state of light through a gain-assisted fast-light medium and detect the remaining quantum correlations. We show that the quantum correlations can be advanced by a small fraction of the correlation time while the entanglement is preserved even in the presence of noise added by phase-insensitive gain. Additionally, although we observe an advance of the peak of the quantum mutual information between the modes, we find that the degradation of the mutual information due to the added noise appears to prevent an advancement of the leading edge. In contrast, we show that both the leading and trailing edges of the mutual information in a slow-light system can be significantly delayed.
We report the generation of a squeezed vacuum state of light whose noise ellipse rotates as a function of the detection frequency. The squeezed state is generated via a four-wave mixing process in a vapor of 85Rb. We observe that rotation varies with
experimental parameters such as pump power and laser detunings. We use a theoretical model based on the Heisenberg-Langevin formalism to describe this effect. Our model can be used to investigate the parameter space and to tailor the ellipse rotation in order to obtain an optimum squeezing angle, for example, for coupling to an interferometer whose optimal noise quadrature varies with frequency.
We show that portions of an image written into a gradient echo memory can be individually retrieved or erased on demand, an important step towards processing a spatially multiplexed quantum signal. Targeted retrieval is achieved by locally addressing
the transverse plane of the storage medium, a warm 85Rb vapor, with a far-detuned control beam. Spatially addressable erasure is similarly implemented by imaging a bright beam tuned near the 85Rb D1 line in order to scatter photons and induce decoherence. Under our experimental conditions atomic diffusion is shown to impose an upper bound on the effective spatial capacity of the memory. The decoherence induced by the optical eraser is characterized and modeled as the response of a two level atom in the presence of a strong driving field.
Using four-wave mixing in a hot atomic vapor, we generate a pair of entangled twin beams in the microsecond pulsed regime near the D1 line of $^{85}$Rb, making it compatible with commonly used quantum memory techniques. The beams are generated in the
bright and vacuum-squeezed regimes, requiring two separate methods of analysis, without and with local oscillators, respectively. We report a noise reduction of up to $3.8pm 0.2$ dB below the standard quantum limit in the pulsed regime and a level of entanglement that violates an Einstein--Podolsky--Rosen inequality.
We experimentally determine the quantum discord present in two-mode squeezed vacuum generated by a four-wave mixing process in hot rubidium vapor. The frequency spectra of the discord, as well as the quantum and classical mutual information are also
measured. In addition, the effects of symmetric attenuation introduced into both modes of the squeezed vacuum on the discord, the quantum mutual information and the classical correlations are examined experimentally. Finally, we show that due to the multi-spatial-mode nature of the four-wave mixing process, the quantum discord may exhibit sub- or superadditivity depending on which spatial channels are selected.
We show that it is possible to estimate the shape of an object by measuring only the fluctuations of a probing field, allowing us to expose the object to a minimal light intensity. This scheme, based on noise measurements through homodyne detection,
is useful in the regime where the number of photons is low enough that direct detection with a photodiode is difficult but high enough such that photon counting is not an option. We generate a few-photon state of multi-spatial-mode vacuum-squeezed twin beams using four-wave mixing and direct one of these twin fields through a binary intensity mask whose shape is to be imaged. Exploiting either the classical fluctuations in a single beam or quantum correlations between the twin beams, we demonstrate that under some conditions quantum correlations can provide an enhancement in sensitivity when estimating the shape of the object.
We study the storage and retrieval of images in a hot atomic vapor using the gradient echo memory protocol. We demonstrate that this technique allows for the storage of multiple spatial modes. We study both spatial and temporal multiplexing by storin
g a sequence of two different images in the atomic vapor. The effect of atomic diffusion on the spatial resolution is discussed and characterized experimentally. For short storage time a normalized cross-correlation between a retrieved image and its input of 88 % is reported.
We study quantum intensity correlations produced using four-wave mixing in a room-temperature rubidium vapor cell. An extensive study of the effect of the various parameters allows us to observe very large amounts of non classical correlations.
This paper reports on photoionisation loading based on ultrafast pulses of singly-ionised strontium ions in a linear Paul trap. We take advantage of an autoionising resonance of Sr neutral atoms to form Sr+ by two-photon absorption of femtosecond pul
ses at a wavelength of 431nm. We compare this technique to electron-bombardment ionisation and observe several advantages of photoionisation. It actually allows the loading of a pure Sr+ ion cloud in a low radio-frequency voltage amplitude regime. In these conditions up to 4x10^4 laser-cooled Sr+ ions were trapped.
