High-resolution measurements of the spatial and temporal evolution of megagauss magnetic fields created in intense short-pulse laser-plasma interactions

A pump-probe polarimetric technique is demonstrated, which provides a complete, temporally and spatially-resolved mapping of the megagauss magnetic fields generated in intense short-pulse laser-plasma interactions. A normally-incident time-delayed probe pulse reflected from its critical surface undergoes a change in its ellipticity according to the magneto-optic Cotton-Mouton effect due to the azimuthal nature of the ambient self-generated megagauss magnetic fields. The temporal resolution of the magnetic field mapping is of the order of the pulsewidth, whereas a spatial resolution of a few microns is achieved by this optical technique. In addition, this technique does not suffer from refraction effects due to the steep plasma density gradients owing to the near-normal incidence of the probe pulse and consequently, higher harmonics of the probe can be employed to penetrate deeper into the plasma to even near-solid densities. The spatial and temporal evolution of the megagauss magnetic fields at the target front as well as at the target rear are presented. The micron-scale resolution of the magnetic field mapping provides valuable information on the filamentary instabilities at the target front, whereas probing the target rear mirrors the highly complex fast electron transport in intense laser-plasma interactions.

Micron-Scale Mapping of Megagauss Magnetic Fields in Petawatt Laser-Solid Interactions

We report spatially and temporally resolved measurements of magnetic fields generated by petawatt laser-solid interactions with high spatial resolution, using optical polarimetry. The polarimetric measurements map the megagauss magnetic field profiles generated by the fast electron currents at the target rear. The magnetic fields at the rear of a 50 $mu$m thick aluminum target exhibit distinct and unambiguous signatures of electron beam filamentation. These results are corroborated by hybrid simulations.

Cross-linked polymers in strain: Structure and anisotropic stress

Molecular dynamic simulation enables one to correlate the evolution of the micro-structure with anisotropic stress when a material is subject to strain. The anisotropic stress due to a constant strain-rate load in a cross-linked polymer is primarily dependent on the mean-square bond length and mean-square bond angle. Excluded volume interactions due to chain stacking and spatial distribution also has a bearing on the stress response. The bond length distribution along the chain is not uniform. Rather, the bond lengths at the end of the chains are larger and uniformly decrease towards the middle of the chain from both ends. The effect is due to the presence of cross-linkers. As with linear polymers, at high density values, changes in mean-square bond length dominates over changes in radius of gyration and end-to-end length. That is, bond deformations dominate over changes in size and shape. A large change in the mean-square bond length reflects in a jump in the stress response. Short-chain polymers more or less behave like rigid molecules. Temperature has a peculiar effect on the response in the sense that even though bond lengths increase with temperature, stress response decreases with increasing temperature. This is due to the dominance of excluded volume effects which result in lower stresses at higher temperatures. At low strain rates, some relaxation in the bond stretch is observed from $epsilon=0.2$ to $epsilon=0.5$. At high strain rates, internal deformation of the chains dominate over their uncoiling leading to a rise in the stress levels.

Structure, molecular dynamics, and stress in a linear polymer under dynamic strain

The structural properties of a linear polymer and its evolution in time have a strong bearing on its anisotropic stress response. The mean-square bond length and mean bond angle are the critical parameters that influence the time-varying stress developed in the polymer. The bond length distribution along the chain is uniform without any abrupt changes at the ends. Among the externally set parameters such as density, temperature, strain rate, and chain length, the density as well as the chain length of the polymer have a significant effect on the stress. At high density values, changes in mean-square bond length dominates over changes in radius of gyration and end-to-end length. In other words, bond deformations dominate as opposed to changes in size and shape. Also, there is a large change in the mean-square bond length that is reflected as a jump in the stress. Beyond a particular value of the chain length, $n = 50$, called the entanglement length, stress-response is found to have distinctly different behavior which we attribute to the entanglement effects. Short chain polymers more or less behave like rigid molecules. There is no significant change in their internal structure when loaded. Further, temperature and rate of loading have a very mild effect on the stress. Besides these new results, we can now explain well known polymeric mechanical behavior under dynamic loading from the point of view of the evolution of the molecular dynamics and the derived structural properties. This could possibly lead to polymer synthesis with desired mechanical behavior.