Optical decoherence studies of Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$

Decoherence of the 795 nm $^3$H$_6$ to $^3$H$_4$ transition in 1%Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ (Tm:YGG) is studied at temperatures as low as 1.2 K. The temperature, magnetic field, frequency, and time-scale (spectral diffusion) dependence of the optical coherence lifetime is measured. Our results show that the coherence lifetime is impacted less by spectral diffusion than other known thulium-doped materials. Photon echo excitation and spectral hole burning methods reveal uniform decoherence properties and the possibility to produce full transparency for persistent spectral holes across the entire 56 GHz inhomogeneous bandwidth of the optical transition. Temperature-dependent decoherence is well described by elastic Raman scattering of phonons with an additional weaker component that may arise from a low density of glass-like dynamic disorder modes (two-level systems). Analysis of the observed behavior suggests that an optical coherence lifetime approaching one millisecond may be possible in this system at temperatures below 1 K for crystals grown with optimized properties. Overall, we find that Tm:YGG has superior decoherence properties compared to other Tm-doped crystals and is a promising candidate for applications that rely on long coherence lifetimes, such as optical quantum memories and photonic signal processing.

Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ materials for spectrally multiplexed quantum memories

We investigate the relevant spectroscopic properties of the 795 nm $^3$H$_6$$leftrightarrow$$^3$H$_4$ transition in 1% Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ at temperatures as low as 1.2 K for optical quantum memories based on persistent spectral tailoring of narrow absorption features. Our measurements reveal that this transition has uniform coherence properties over a 56 GHz bandwidth, and a simple hyperfine structure split by $pm$44 MHz/T with lifetimes of up to hours. Furthermore, we find a $^3$F$_4$ population lifetime of 64 ms -- one of the longest lifetimes observed for an electronic level in a solid --, and an exceptionally long coherence lifetime of 490 $mu$s -- the longest ever observed for optical transitions of Tm$^{3+}$ ions in a crystal. Our results suggest that this material allows realizing broadband quantum memories that enable spectrally multiplexed quantum repeaters.

An integrated processor for photonic quantum states using a broadband light-matter interface

Faithful storage and coherent manipulation of quantum optical pulses are key for long distance quantum communications and quantum computing. Combining these functions in a light-matter interface that can be integrated on-chip with other photonic quantum technologies, e.g. sources of entangled photons, is an important step towards these applications. To date there have only been a few demonstrations of coherent pulse manipulation utilizing optical storage devices compatible with quantum states, and that only in atomic gas media (making integration difficult) and with limited capabilities. Here we describe how a broadband waveguide quantum memory based on the Atomic Frequency Comb (AFC) protocol can be used as a programmable processor for essentially arbitrary spectral and temporal manipulations of individual quantum optical pulses. Using weak coherent optical pulses at the few photon level, we experimentally demonstrate sequencing, time-to-frequency multiplexing and demultiplexing, splitting, interfering, temporal and spectral filtering, compressing and stretching as well as selective delaying. Our integrated light-matter interface offers high-rate, robust and easily configurable manipulation of quantum optical pulses and brings fully practical optical quantum devices one step closer to reality. Furthermore, as the AFC protocol is suitable for storage of intense light pulses, our processor may also find applications in classical communications.

Spectral multiplexing for scalable quantum photonics using an atomic frequency comb quantum memory and feed-forward control

Future multi-photon applications of quantum optics and quantum information science require quantum memories that simultaneously store many photon states, each encoded into a different optical mode, and enable one to select the mapping between any input and a specific retrieved mode during storage. Here we show, with the example of a quantum repeater, how to employ spectrally-multiplexed states and memories with fixed storage times that allow such mapping between spectral modes. Furthermore, using a Ti:Tm:LiNbO3 waveguide cooled to 3 Kelvin, a phase modulator, and a spectral filter, we demonstrate storage followed by the required feed-forward-controlled frequency manipulation with time-bin qubits encoded into up to 26 multiplexed spectral modes and 97% fidelity.

Conditional detection of pure quantum states of light after storage in a waveguide

Conditional detection is an important tool to extract weak signals from a noisy background and is closely linked to heralding, which is an essential component of protocols for long distance quantum communication and distributed quantum information processing in quantum networks. Here we demonstrate the conditional detection of time-bin qubits after storage in and retrieval from a photon-echo based waveguide quantum memory. Each qubit is encoded into one member of a photon-pair produced via spontaneous parametric down conversion, and the conditioning is achieved by the detection of the other member of the pair. Performing projection measurements with the stored and retrieved photons onto different bases we obtain an average storage fidelity of 0.885 pm 0.020, which exceeds the relevant classical bounds and shows the suitability of our integrated light-matter interface for future applications of quantum information processing.