The analytical expressions for the time-dependent cross-correlations of the translational and rotational Brownian displacements of a particle with arbitrary shape are derived. The reference center is arbitrary, and the reference frame is such that th
e rotational-rotational diffusion tensor is diagonal.
Dynamics of flexible non-Brownian fibers in shear flow at low-Reynolds-number are analyzed numerically for a wide range of the ratios A of the fiber bending force to the viscous drag force. Initially, the fibers are aligned with the flow, and later t
hey move in the plane perpendicular to the flow vorticity. A surprisingly rich spectrum of different modes is observed when the value of A is systematically changed, with sharp transitions between coiled and straightening out modes, period-doubling bifurcations from periodic to migrating solutions, irregular dynamics and chaos.
Brownian motion of a particle with an arbitrary shape is investigated theoretically. Analytical expressions for the time-dependent cross-correlations of the Brownian translational and rotational displacements are derived from the Smoluchowski equatio
n. The role of the particle mobility center is determined and discussed.
Dynamics of regular clusters of many non-touching particles falling under gravity in a viscous fluid at low Reynolds number are analysed within the point-particle model. Evolution of two families of particle configurations is determined: 2 or 4 regul
ar horizontal polygons (called `rings) centred above or below each other. Two rings fall together and periodically oscillate. Four rings usually separate from each other with chaotic scattering. For hundreds of thousands of initial configurations, a map of the cluster lifetime is evaluated, where the long-lasting clusters are centred around periodic solutions for the relative motions, and surrounded by regions of the chaotic scattering,in a similar way as it was observed by Janosi et al. (1997) for three particles only. These findings suggest to consider the existence of periodic orbits as a possible physical mechanism of the existence of unstable clusters of particles falling under gravity in a viscous fluid.
We use numerical simulations of a bead-spring model chain to investigate the evolution of the conformation of long and flexible elastic fibers in a steady shear flow. In particular, for rather open initial configurations, and by varying a dimensionle
ss elastic parameter, we identify two distinct conformational modes with different final size, shape, and orientation. Through further analysis we identify slipknots in the chain. Finally, we provide examples of initial configurations of an open trefoil knot that the flow unknots and then knots again, sometimes repeating several times. These changes in topology should be reflected in changes in bulk rheological and/or transport properties.
Hydrodynamic interactions between two identical elastic dumbbells settling under gravity in a viscous fluid at low-Reynolds-number are investigated within the point-particle model. Evolution of a benchmark initial configuration is studied, in which t
he dumbbells are vertical and their centres are aligned horizontally. Rigid dumbbells and pairs of separate beads starting from the same positions tumble periodically while settling down. We find that elasticity (which breaks time-reversal symmetry of the motion) significantly affects the systems dynamics. This is remarkable taking into account that elastic forces are always much smaller than gravity. We observe oscillating motion of the elastic dumbbells, which tumble and change their length non-periodically. Independently of the value of the spring constant, a horizontal hydrodynamic repulsion appears between the dumbbells - their centres of mass move apart from each other horizontally. The shift is fast for moderate values of the spring constant k, and slows down when k tends to zero or to infinity; in these limiting cases we recover the periodic dynamics reported in the literature. For moderate values of the spring constant, and different initial configurations, we observe the existence of a universal time-dependent solution to which the system converges after an initial relaxation phase. The tumbling time and the width of the trajectories in the centre-of-mass frame increase with time. In addition to its fundamental significance, the benchmark solution presented here is important to understand general features of systems with larger number of elastic particles, at regular and random configurations.
Systems of spherical particles moving in Stokes flow are studied for a different particle internal structure and boundaries, including the Navier-slip model. It is shown that their hydrodynamic interactions are well described by treating them as soli
d spheres of smaller hydrodynamic radii, which can be determined from measured single-particle diffusion or intrinsic viscosity coefficients. Effective dynamics of suspensions made of such particles is quite accurately described by mobility coefficients of the solid particles with the hydrodynamic radii, averaged with the unchanged direct interactions between the particles.
We investigate regular configurations of a small number of particles settling under gravity in a viscous fluid. The particles do not touch each other and can move relative to each other. The dynamics is analyzed in the point-particle approximation. A
family of regular configurations is found with periodic oscillations of all the settling particles. The oscillations are shown to be robust under some out-of-phase rearrangements of the particles. In the presence of an additional particle above such a regular configuration, the particle periodic trajectories are horizontally repelled from the symmetry axis, and flattened vertically. The results are used to propose a mechanism how a spherical cloud, made of a large number of particles distributed at random, evolves and destabilizes.
For suspensions of permeable particles, the short-time translational and rotational self-diffusion coefficients, and collective diffusion and sedimentation coefficients are evaluated theoretically. An individual particle is modeled as a uniformly per
meable sphere of a given permeability, with the internal solvent flow described by the Debye-Bueche-Brinkman equation. The particles are assumed to interact non-hydrodynamically by their excluded volumes. The virial expansion of the transport properties in powers of the volume fraction is performed up to the two-particle level. The first-order virial coefficients corresponding to two-body hydrodynamic interactions are evaluated with very high accuracy by the series expansion in inverse powers of the inter-particle distance. Results are obtained and discussed for a wide range of the ratio, x, of the particle radius to the hydrodynamic screening length inside a permeable sphere. It is shown that for x >= 10, the virial coefficients of the transport properties are well-approximated by the hydrodynamic radius (annulus) model developed by us earlier for the effective viscosity of porous-particle suspensions.
