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59 - O. Breunig , M. Garst , A. Rosch 2014
In this study the magnetic order of the spin-1/2 XXZ chain system Cs$_2$CoCl$_4$ in a temperature range from 50 mK to 0.5 K and in applied magnetic fields up to 3.5 T is investigated by high-resolution measurements of the thermal expansion and the sp ecific heat. Applying magnetic fields along a or c suppresses $T_textrm{N}$ completely at about 2.1 T. In addition, we find an adjacent intermediate phase before the magnetization saturates close to 2.5 T. For magnetic fields applied along b, a surprisingly rich phase diagram arises. Two additional transitions are observed at critical fields $mu_0 H_{SF1}simeq 0.25$ T and $mu_0 H_{SF2}simeq 0.7$ T, which we propose to arise from a two-stage spin-flop transition.
99 - O. Breunig , M. Garst , E. Sela 2013
Comparing high-resolution specific heat and thermal expansion measurements to exact finite-size diagonalization, we demonstrate that Cs$_2$CoCl$_4$ for a magnetic field along the crystallographic b axis realizes the spin-$frac{1}{2}$ XXZ chain in a t ransverse field. Exploiting both thermal as well as virtual excitations of higher crystal field states, we find that the spin chain is in the XY-limit with an anisotropy $J_z/J_perp approx 0.12$ substantially smaller than previously believed. A spin-flop Ising quantum phase transition occurs at a critical field of $mu_0 H_b^{rm cr} approx 2$ T before around 3.5 T the description in terms of an effective spin-$frac{1}{2}$ chain becomes inapplicable.
Bicritical points, at which two distinct symmetry-broken phases become simultaneously unstable, are typical for spin-flop metamagnetism. Interestingly, the heavy-fermion compound YbAgGe also possesses such a bicritical point (BCP) with a low temperat ure T_BCP ~ 0.3 K at a magnetic field of mu_0 H_BCP ~ 4.5 T. In its vicinity, YbAgGe exhibits anomalous behavior that we attribute to the influence of a quantum bicritical point (QBCP), that is close in parameter space yet can be reached by tuning T_BCP further to zero. Using high-resolution measurements of the magnetocaloric effect, we demonstrate that the magnetic Grueneisen parameter Gamma_H indeed both changes sign and diverges as required for quantum criticality. Moreover, Gamma_H displays a characteristic scaling behavior but only on the low-field side, H < H_BCP, indicating a pronounced asymmetry with respect to the critical field. We speculate that the small value of T_BCP is related to the geometric frustration of the Kondo-lattice of YbAgGe.
98 - T. Lorenz , O. Heyer , M. Garst 2008
We present high-resolution measurements of the $c^star$-axis thermal expansion and magnetostriction of piperidinium copper bromide hp. The experimental data at low temperatures is well accounted for by a two-leg spin-ladder Hamiltonian. The thermal e xpansion shows a complex behaviour with various sign changes and approaches a $1/sqrt{T}$ divergence at the critical fields. All low-temperature features are semi-quantitatively explained within a free fermion model; full quantitative agreement is obtained with Quantum Monte Carlo simulations.
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