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224 - M. Wurdack , E. Estrecho , S. Todd 2021
Atomically-thin transition metal dichalcogenide crystals (TMDCs) hold great promise for future semiconductor optoelectronics due to their unique electronic and optical properties. In particular, electron-hole pairs (excitons) in TMDCs are stable at r oom temperature and interact strongly with light. When TMDCs are embedded in an optical microcavity, the excitons can hybridise with cavity photons to form exciton polaritons (polaritons herein), which display both ultrafast velocities and strong interactions. The ability to manipulate and trap polaritons on a microchip is critical for future applications. Here, we create a potential landscape for room-temperature polaritons in monolayer WS$_2$, and demonstrate their free propagation and trapping. We show that the effect of dielectric disorder, which restricts the diffusion of WS$_2$ excitons and broadens their spectral resonance, is dramatically reduced in the strong exciton-photon coupling regime leading to motional narrowing. This enables the ballistic transport of WS$_2$ polaritons across tens of micrometers with an extended range of partial first-order coherence. Moreover, the dephasing of trapped polaritons is dramatically suppressed compared to both WS$_2$ excitons and free polaritons. Our results demonstrate the possibility of long-range transport and efficient trapping of TMDC polaritons in ambient conditions.
We report the observation of low-energy, low-momenta collective oscillations of an excitonpolariton condensate in a round box trap. The oscillations are dominated by the dipole and breathing modes, and the ratio of the frequencies of the two modes is consistent with that of a weakly interacting two-dimensional trapped Bose gas. The speed of sound extracted from the dipole oscillation frequency is smaller than the Bogoliubov sound, which can be partly explained by the influence of the incoherent reservoir. These results pave the way for understanding the effects of reservoir, dissipation, energy relaxation, and finite temperature on the superfluid properties of exciton-polariton condensates and other two-dimensional open-dissipative quantum fluids.
Intense X-ray free-electron lasers (XFELs) can rapidly excite matter, leaving it in inherently unstable states that decay on femtosecond timescales. As the relaxation occurs primarily via Auger emission, excited state observations are constrained by Auger decay. In situ measurement of this process is therefore crucial, yet it has thus far remained elusive at XFELs due to inherent timing and phase jitter, which can be orders of magnitude larger than the timescale of Auger decay. Here, we develop a new approach termed self-referenced attosecond streaking, based upon simultaneous measurements of streaked photo- and Auger electrons. Our technique enables sub-femtosecond resolution in spite of jitter. We exploit this method to make the first XFEL time-domain measurement of the Auger decay lifetime in atomic neon, and, by using a fully quantum-mechanical description, retrieve a lifetime of $2.2^{ + 0.2}_{ - 0.3}$ fs for the KLL decay channel. Importantly, our technique can be generalised to permit the extension of attosecond time-resolved experiments to all current and future FEL facilities.
100 - G. Arnold , M. Wulf , S. Barzanjeh 2020
Practical quantum networks require low-loss and noise-resilient optical interconnects as well as non-Gaussian resources for entanglement distillation and distributed quantum computation. The latter could be provided by superconducting circuits but - despite growing efforts and rapid progress - existing solutions to interface the microwave and optical domains lack either scalability or efficiency, and in most cases the conversion noise is not known. In this work we utilize the unique opportunities of silicon photonics, cavity optomechanics and superconducting circuits to demonstrate a fully integrated, coherent transducer connecting the microwave X and the telecom S bands with a total (internal) bidirectional transduction efficiency of 1.2% (135 %) at millikelvin temperatures. The coupling relies solely on the radiation pressure interaction mediated by the femtometer-scale motion of two silicon nanobeams and includes an optomechanical gain of about 20 dB. The chip-scale device is fabricated from CMOS compatible materials and achieves a V$_pi$ as low as 16 $mu$V for sub-nanowatt pump powers. Such power-efficient, ultra-sensitive and highly integrated hybrid interconnects might find applications ranging from quantum communication and RF receivers to magnetic resonance imaging.
Competing magnetic interactions in geometrically frustrated magnets give rise to new forms of correlated matter, such as spin liquids and spin ices. Characterizing the magnetic structure of these states has been difficult due to the absence of long-r ange order. Here, we demonstrate that the spin Seebeck effect (SSE) is a sensitive probe of magnetic short-range order (SRO) in geometrically frustrated magnets. In low temperature (2 - 5 K) SSE measurements on a model frustrated magnet mathrm{Gd_{3}Ga_{5}O_{12}}, we observe modulations in the spin current on top of a smooth background. By comparing to existing neutron diffraction data, we find that these modulations arise from field-induced magnetic ordering that is short-range in nature. The observed SRO is anisotropic with the direction of applied field, which is verified by theoretical calculation.
A combined analysis of x-ray absorption and resonant reflectivity data was used to obtain the orbital polarization profiles of superlattices composed of four-unit-cell-thick layers of metallic LaNiO3 and layers of insulating RXO3 (R=La, Gd, Dy and X= Al, Ga, Sc), grown on substrates that impose either compressive or tensile strain. This superlattice geometry allowed us to partly separate the influence of epitaxial strain from interfacial effects controlled by the chemical composition of the insulating blocking layers. Our quantitative analysis reveal orbital polarizations up to 25%. We further show that strain is the most effective control parameter, whereas the influence of the chemical composition of the blocking layers is comparatively small.
110 - J. R. Ott , M. Wubs , P. Lodahl 2013
We investigate cooperative fluorescence in a dilute cloud of strongly driven two-level emitters. Starting from the Heisenberg equations of motion, we compute the first-order scattering corrections to the saturation of the excited-state population and to the resonance-fluorescence spectrum, which both require going beyond the state-of-the-art linear-optics approach to describe collective phenomena. A dipole blockade is observed due to long range dipole-dipole coupling that vanishes at stronger driving fields. Furthermore, we compute the inelastic component of the light scattered by a cloud of many atoms and find that the Mollow triplet is affected by cooperativity. In a lobe around the forward direction, the inelastic Mollow triplet develops a spectral asymmetry, observable under experimental conditions.
Magnetoelectric susceptibility of a metamaterial built from split ring resonators have been investigated both experimentally and within an equivalent circuit model. The absolute values have been shown to exceed by two orders of magnitude that of clas sical magnetoelectric materials. The metamaterial investigated reaches the theoretically predicted value of the magnetoelectric susceptibility which is equal to the geometric average of the electric and magnetic susceptibilities.
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