Photoinduced Kerr rotation by more than $pi /2$ radians is demonstrated in planar quantum well microcavity in the strong coupling regime. This result is close to the predicted theoretical maximum of $pi $. It is achieved by engineering microcavity pa
rameters such that the optical impedance matching condition is reached at the smallest negative detuning between exciton resonance and the cavity mode. This ensures the optimum combination of the exciton induced optical non-linearity and the enhancement of the Kerr angle by the cavity. Comprehensive analysis of the polarization state of the light in this regime shows that both renormalization of the exciton energy and the saturation of the excitonic resonance contribute to the observed optical nonlinearities.
Highly polarized nuclear spins within a semiconductor quantum dot (QD) induce effective magnetic (Overhauser) fields of up to several Tesla acting on the electron spin or up to a few hundred mT for the hole spin. Recently this has been recognized as
a resource for intrinsic control of QD-based spin quantum bits. However, only static long-lived Overhauser fields could be used. Here we demonstrate fast redirection on the microsecond time-scale of Overhauser fields of the order of 0.5 T experienced by a single electron spin in an optically pumped GaAs quantum dot. This has been achieved using full coherent control of an ensemble of 10^3-10^4 optically polarized nuclear spins by sequences of short radio-frequency (rf) pulses. These results open the way to a new class of experiments using rf techniques to achieve highly-correlated nuclear spins in quantum dots, such as adiabatic demagnetization in the rotating frame leading to sub-micro K nuclear spin temperatures, rapid adiabatic passage, and spin squeezing.
We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically forbidden transitions. This process corresponds to one-to-one conversion of a photon absorbed by the d
ot into a polarized nuclear spin, which also has potential for initialization of hole spin in QDs. Pumping via the forbidden transition is a manifestation of the optical solid effect, an optical analogue of the effect previously observed in electron spin resonance experiments in the solid state. We find that by employing this effect, nuclear polarization of 65% can be achieved, the highest reported so far in optical orientation studies in QDs. The efficiency of the spin pumping exceeds that employing the allowed transition, which saturates due to the low probability of electron-nuclear spin flip-flop.
We report a surprisingly long spin relaxation time of electrons in Mn-doped p-GaAs. The spin relaxation time scales with the optical pumping and increases from 12 ns in the dark to 160 ns upon saturation. This behavior is associated with the differen
ce in spin relaxation rates of electrons precessing in the fluctuating fields of ionized or neutral Mn acceptors, respectively. For the latter the antiferromagnetic exchange interaction between a Mn ion and a bound hole results in a partial compensation of these fluctuating fields, leading to the enhanced spin memory.
We study bound magnetic polarons (BMP) in a very diluted magnetic semiconductor CdMnTe by means of site selective spectroscopy. In zero magnetic field we detect a broad and asymmetric band with a characteristic spectral width of about 5 meV. When ext
ernal magnetic fields are applied a new line appears in the emission spectrum. Remarkably, the spectral width of this line is reduced greatly down to 0.24 meV. We attribute such unusual behavior to the formation of BMP, effected by sizable fluctuations of local magnetic moments. The modifications of the optical spectra have been simulated by the Monte-Carlo method and calculated within an approach considering the nearest Mn ion. A quantitative agreement with the experiment is achieved without use of fitting parameters. It is demonstrated that the low-energy part of the emission spectra originates from the energetic relaxation of a complex consisting of a hole and its nearest Mn ion. It is also shown that the contribution to the narrow line arises from the remote Mn ions.
