We present muon spin lattice relaxation measurements in the V15 spin 1/2 molecular nano-magnet. We find that the relaxation rate in low magnetic fields (<5 kG) is temperature independent below ~10 K, implying that the molecular spin is dynamically fl
uctuating down to 12 mK. These measurements show that the fluctuation time increases as the temperature is decreased and saturates at a value of ~6 nsec at low temperatures. The fluctuations are attributed to V15 molecular spin dynamics perpendicular to the applied magnetic field direction, induced by coupling between the molecular spin and nuclear spin bath in the system.
The magnetic properties of a monolayer of Mn12 single molecule magnets grafted onto a Si substrate have been investigated using depth-controlled $beta$-detected nuclear magnetic resonance. A low energy beam of spin polarized radioactive 8Li was used
to probe the local static magnetic field distribution near the Mn12 monolayer in the Si substrate. The resonance linewidth varies strongly as a function of implantation depth as a result of the magnetic dipolar fields generated by the Mn12 electronic magnetic moments. The temperature dependence of the linewidth indicates that the magnetic properties of the Mn12 moments in this low dimensional configuration differ from bulk Mn12.
