Although nuclear fission can be understood qualitatively as an evolution of the nuclear shape, a quantitative description has proven to be very elusive. In particular, until now, there exists no model with demonstrated predictive power for the fissio
n fragment mass yields. Exploiting the expected strongly damped character of nuclear dynamics, we treat the nuclear shape evolution in analogy with Brownian motion and perform random walks on five-dimensional fission potential-energy surfaces which were calculated previously and are the most comprehensive available. Test applications give good reproduction of highly variable experimental mass yields. This novel general approach requires only a single new global parameter, namely the critical neck size at which the mass split is frozen in, and the results are remarkably insensitive to its specific value.
The spinodal amplification of density fluctuations is treated perturbatively within dissipative fluid dynamics for the purpose of elucidating the prospects for this mechanism to cause a phase separation to occur during a relativistic nuclear collisio
n. The present study includes not only viscosity but also heat conduction (whose effect on the growth rates is of comparable magnitude but opposite), as well as a gradient term in the local pressure, and the corresponding dispersion relation for collective modes in bulk matter is derived from relativistic fluid dynamics. A suitable two-phase equation of state is obtained by interpolation between a hadronic gas and a quark-gluon plasma, while the transport coefficients are approximated by simple parametrizations that are suitable at any degree of net baryon density. We calculate the degree of spinodal amplification occurring along specific dynamical phase trajectories characteristic of nuclear collision at various energies. The results bring out the important fact that the prospects for spinodal phase separation to occur can be greatly enhanced by careful tuning of the collision energy to ensure that the thermodynamic conditions associated with the maximum compression lie inside the region of spinodal instability.
We construct a simple two-phase equation of state intended to resemble that of compressed baryon-rich matter and then introduce a gradient term in the compressional energy density to take account of fintie-range effects in non-uniform configurations.
With this model we study the interface between the two coexisting phases and obtain estimates for the associated interface tension. Subsequently, we incorporate the finite-range equation of state into ideal or viscous fluid dynamics and derive the collective dispersion relation for the mechanically unstable modes of bulk matter in the spinodal region of the thermodynamic phase diagram. Combining these results with time scales extracted from existing dynamical transport simulations, we discuss the prospects for spinodal phase separation to occur in nuclear collisions. We argue that these can be optimized by a careful tuning of the collision energy to maximize the time spent by the bulk of the system inside the mechanically unstable spinodal region of the phase diagram. Our specific numerical estimates suggest cautious optimism that this phenomenon may in fact occur, though a full dynamical simulation is needed for a detailed assessment.
