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Topological semimetals are systems in which the conduction and the valence bands cross each other and this crossing is protected by topological constraints. These materials provide an intriguing test of fundamental theory and their exceptional physic al properties promise a wide range of possible applications. Here we report a study of the thermoelectric power (S) for a single crystal of ZrSiS that is believed to be a topological nodal-line semimetal. We detect multiple quantum oscillations in the magnetic field dependence of S that are still visible at temperature as high as T = 100 K. Two of these oscillation frequencies are shown to arise from 3D and 2D bands, each with linear dispersion and the additional Berry phase expected theoretically.
We report measurements of the magnetic susceptibility of twinned single crystals of YBa$_{2}$Cu$_{3}$O$_{6+x}$ from just above their superconducting transition temperatures to 300 K with magnetic fields of up to 5 T applied parallel and perpendicular to the CuO$_2$ planes at 7 values of $x$. Appropriate analysis allows the relatively small, but still important, Curie terms to be separated from other contributions to the susceptibility. Our data support a picture in which the Curie terms arise from oxygen disorder in the Cu-O chains. This agrees with published work on polycrystalline samples where the sample cooling rate was varied, but here we show that the Curie plots flatten out above 200 K. We identify small effects of charge density wave (CDW) instabilities in the temperature ($T$) derivative of the in-plane susceptibility $dchi_{ab}(T)/dT$ and discuss their $x$-dependence. For $x=$0.67 we make a detailed comparison with published high energy X-ray diffraction data using a minimal model involving Fermi arcs, thereby obtaining values for the CDW energy gap and the Helmholtz free energy in a coherence volume. At 80 and 100 K the latter is comparable with, or smaller than $k_BT$ respectively, highlighting the probable importance of thermal fluctuations. We note that the effect of the Lorentz force on charge carriers in the Fermi arcs could provide a simple mechanism for enhancing the CDWs in high magnetic fields, as suggested by recent experiments.
We report intrinsic tunnelling data for mesa structures fabricated on three over- and optimally-doped $rm{Bi_{2.15}Sr_{1.85}CaCu_{2}O_{8+delta}}$ crystals with transition temperatures of 86-78~K and 0.16-0.19~holes per CuO$_2$ unit, for a wide range of temperature ($T$) and applied magnetic field ($H$), primarily focusing on one over-doped crystal(OD80). The differential conductance above the gap edge shows clear dip structure which is highly suggestive of strong coupling to a narrow boson mode. Data below the gap edge suggest that tunnelling is weaker near the nodes of the d-wave gap and give clear evidence for strong $T$-dependent pair breaking. These findings could help theorists make a detailed Eliashberg analysis and thereby contribute towards understanding the pairing mechanism. We show that for our OD80 crystal the gap above $T_c$ although large, is reasonably consistent with the theory of superconducting fluctuations.
We report measurements of the thermoelectric power (TEP) for a series of Pb(1-x)Tl(x)Te crystals with x = 0.0 to 1.3%. Although the TEP is very large for x = 0.0, using a single band analysis based on older work for dilute magnetic alloys we do find evidence for a Kondo contribution of 11 - 18 uV/K. This analysis suggests that Tk is ~ 50 - 70 K, a factor 10 higher than previously thought.
We report Nernst effect measurements for some crystalline films of Ca and Zn-doped yttrium barium copper oxide grown by pulsed laser deposition. We argue that our results and most of the published data for LSCO are consistent with the theory of Gaussian superconducting fluctuations.
35 - J.R. Cooper 2007
The results of a computer analysis of a simple 2D quantum mechanical tunnelling model are reported. These suggest that the spatial dependence of the superconducting energy gap observed by Scanning Tunnelling Spectroscopy (STS) studies of single cryst als of the high Tc superconductor Bi:2212 is not necessarily caused by nanoscale inhomogeneity. Instead the spatial dependence of the STS data could arise from the momentum (k) dependence of the energy gap, which is a defining feature of a d-wave superconductor. It is possible that this viewpoint could be exploited to obtain k-dependent information from STS studies.
We report a de Haas-van Alphen (dHvA) study of the electronic structure of Al doped crystals of MgB$_2$. We have measured crystals with $sim 7.5$% Al which have a $T_c$ of 33.6 K, ($sim 14$% lower than pure MgB$_2$). dHvA frequencies for the $sigma$ tube orbits in the doped samples are lower than in pure MgB$_2$, implying a $16pm2%$ reduction in the number of holes in this sheet of Fermi surface. The mass of the quasiparticles on the larger $sigma$ orbit is lighter than the pure case indicating a reduction in electron-phonon coupling constant $lambda$. These observations are compared with band structure calculations, and found to be in excellent agreement.
A universal scaling relation, $rho_s propto sigma(T_c)times T_c$ has been reported by Homes $et$ $al$. (Nature (London) {bf 430}, 539 (2004)) where $rho_s$ is the superfluid density and $sigma(T)$ is the DC conductivity. The relation was shown to app ly to both c-axis and in-plane dynamics for high-$T_c$ superconductors as well as to the more conventional superconductors Nb and Pb, suggesting common physics in these systems. We show quantitatively that the scaling behavior has several possible origins including, marginal Fermi-liquid behavior, Josephson coupling, dirty-limit superconductivity and unitary impurity scattering for a d-wave order parameter. However, the relation breaks down seriously in overdoped cuprates, and possibly even at lower doping.
We report measurements of the de Haas-van Alphen effect for single crystals of MgB$_2$, in magnetic fields up to 32 Tesla. In contrast to our earlier work, dHvA orbits from all four sheets of the Fermi surface were detected. Our results are in good o verall agreement with calculations of the electronic structure and the electron-phonon mass enhancements of the various orbits, but there are some small quantitative discrepancies. In particular, systematic differences in the relative volumes of the Fermi surface sheets and the magnitudes of the electron-phonon coupling constants could be large enough to affect detailed calculations of T$_{c}$ and other superconducting properties.
We report observations of quantum oscillations in single crystals of the high temperature superconductor MgB_2. Three de Haas-van Alphen frequencies are clearly resolved. Comparison with band structure calculations strongly suggests that two of these come from a single warped Fermi surface tube along the c direction, and that the third arises from cylindrical sections of an in-plane honeycomb network. The measured values of the effective mass range from 0.44-0.68 m_e. By comparing these with band masses calculated recently by three groups, we find that the electron-phonon coupling strength lambda, is a factor ~3 larger for the c-axis tube orbits than for the in-plane network orbit, in accord with recent microscopic calculations.
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