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By means of electron spin resonance investigations we revealed the crucial role of the interchain coupling in the spin dynamics of the spin-1/2 Heisenberg antiferromagnetic (AF) chain material copper-pyrazine-dinitrate, Cu(C$_4$H$_4$N$_2$)(NO$_3$)$_2 $. We found that the dominating interchain interaction is of a zig-zag type. This interaction gives rise to geometrical frustration effects and strongly influences the character of AF ordering. Combining our experimental findings with the results of a quasiclassical approach we argue that at low temperatures the system orders in an incommensurate spiral state.
Magnetic excitations in the spin-ladder material (C$_5$H$_{12}$N)$_2$CuBr$_4$ [BPCB] are probed by high-resolution multi-frequency electron spin resonance (ESR) spectroscopy. Our experiments provide a direct evidence for a biaxial anisotropy ($sim 5% $ of the dominant exchange interaction), that is in contrast to a fully isotropic spin-ladder model employed for this system previously. It is argued that this anisotropy in BPCB is caused by spin-orbit coupling, which appears to be important for describing magnetic properties of this compound. The zero-field zone-center gap in the excitation spectrum of BPCB, $Delta_0/k_{B}=16.5$ K, is detected directly. Furthermore, an ESR signature of the inter-ladder exchange interactions is obtained. The detailed characterization of the anisotropy in BPCB completes the determination of the full spin hamiltonian of this exceptional spin-ladder material and shows ways to study anisotropy effects in spin ladders.
We have measured the complex dynamical conductivity, $sigma = sigma_{1} + isigma_{2}$, of superconducting Ba(Fe$_{0.9}$Co$_{0.1}$)$_{2}$As$_{2}$ ($T_{c} = 22$ K) at terahertz frequencies and temperatures 2 - 30 K. In the frequency dependence of $sigm a_{1}$ below $T_{c}$, we observe clear signatures of the superconducting energy gap opening. The temperature dependence of $sigma_{1}$ demonstrates a pronounced coherence peak at frequencies below 15 cm$^{-1}$ (1.8 meV). The temperature dependence of the penetration depth, calculated from $sigma_{2}$, shows power-law behavior at the lowest temperatures. Analysis of the conductivity data with a two-gap model, gives the smaller isotropic s-wave gap of $Delta_{A} = 3$ meV, while the larger gap is highly anisotropic with possible nodes and its rms amplitude is $Delta_{0} = 8$ meV. Overall, our results are consistent with a two-band superconductor with an $s_{pm}$ gap symmetry.
$Ni Cl_2$-$4SC(NH_2)_2$ (known as DTN) is a spin-1 material with a strong single-ion anisotropy that is regarded as a new candidate for Bose-Einstein condensation (BEC) of spin degrees of freedom. We present a systematic study of the low-energy excit ation spectrum of DTN in the field-induced magnetically ordered phase by means of high-field electron spin resonance measurements at temperatures down to 0.45 K. We argue that two gapped modes observed in the experiment can be consistently interpreted within a four-sublattice antiferromagnet model with a finite interaction between two tetragonal subsystems and unbroken axial symmetry. The latter is crucial for the interpretation of the field-induced ordering in DTN in terms of BEC.
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