Ferromagnet/Superconductor/Ferromagnet (F/S/F) trilayers constitute the core of a superconducting spin valve. The switching effect of the spin valve is based on interference phenomena occurring due to the proximity effect at the S/F interfaces. A rem
arkable effect is only expected if the core structure exhibits strong critical temperature oscillations, or most favorable, reentrant superconductivity, when the thickness of the ferromagnetic layer is increased. The core structure has to be grown on an antiferromagnetic oxide layer (or such layer to be placed on top) to pin by exchange bias the magnetization-orientation of one of the ferromagnetic layers. In the present paper we demonstrate that this is possible, keeping the superconducting behavior of the core structure undisturbed.
The upper critical magnetic field H_{c2} in thin-film FSF trilayer spin-valve cores is studied experimentally and theoretically in geometries perpendicular and parallel to the heterostructure surface. The series of samples with variable thicknesses o
f the bottom and of the top Cu_{41}Ni_{59} F-layers are prepared in a single run, utilizing a wedge deposition technique. The critical field H_{c2} is measured in the temperature range $0.4-8$ K and for magnetic fields up to 9 Tesla. A transition from oscillatory to reentrant behavior of the superconducting transition temperature versus F-layers thickness, induced by an external magnetic field, has been observed for the first time. In order to properly interpret the experimental data, we develop a quasiclassical theory, enabling one to evaluate the temperature dependence of the critical field and the superconducting transition temperature for an arbitrary set of the system parameters. A fairly good agreement between our experimental data and theoretical predictions is demonstrated for all samples, using a single set of fit parameters. This confirms adequacy of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) physics in determining the unusual superconducting properties of the studied Cu_{41}Ni_{59}/Nb/Cu_{41}Ni_{59} spin-valve core trilayers.
The theory of superconductor-ferromagnet (S-F) heterostructures with two ferromagnetic layers predicts the generation of a long-range, odd-in-frequency triplet pairing at non-collinear alignment (NCA) of the magnetizations of the F-layers. This tripl
et pairing has been detected in a Nb/Cu41Ni59/nc-Nb/Co/CoOx spin-valve type proximity effect heterostructure, in which a very thin Nb film between the F-layers serves as a normal conducting (nc) spacer. The resistance of the sample as a function of an external magnetic field shows that for not too high fields the system is superconducting at a collinear alignment of the Cu41Ni59 and Co layer magnetic moments, but switches to the normal conducting state at a NCA configuration. This indicates that the superconducting transition temperature Tc for NCA is lower than the fixed measuring temperature. The existence of a minimum Tc, at the NCA regime below that one for parallel or antiparallel alignments of the F-layer magnetic moments, is consistent with the theoretical prediction of a singlet superconductivity suppression by the long-range triplet pairing generation.
Ferromagnet/Superconductor/Ferromagnet (F/S/F) trilayers, in which the establishing of a Fulde-Ferrell Larkin-Ovchinnikov (FFLO) like state leads to interference effects of the superconducting pairing wave function, form the core of the superconducti
ng spin valve. The realization of strong critical temperature oscillations in such trilayers, as a function of the ferromagnetic layer thicknesses or, even more efficient, reentrant superconductivity, are the key condition to obtain a large spin valve effect, i.e. a large shift in the critical temperature. Both phenomena have been realized experimentally in the Cu 41 Ni 59 /Nb/Cu 41 Ni 59 trilayers investigated in the present work.
The theoretical description of the Fulde-Ferrell-Larkin-Ovchinnikov like state establishing in nanostructered bilayers of ferromagnetic (F) and superconducting (S) material leads to critical temperature oscillations and reentrant superconductivity as
the F-layer thickness gradually increases. The experimental realization of these phenomena is an important prerequisite for the fabrication of the Ferromagnet/Superconductor/Ferromagnet core structure of the superconducting spin-valve. A switching of the spin-valve is only expected if such non-monotonic critical temperature behavior is observed in F/S bilayers as well as in the S/F bilayers, a combination of which the spin-valve core structure can be regarded to consist of. In our former investigations we could demonstrate the required non-monotonic behavior of the critical temperature in S/F bilayers. In this study we succeeded in the preparation of F/S bilayers, where the superconducting material is now grown on top of the ferromagnetic metal, which show deep critical temperature oscillations as a function of the ferromagnetic layer thickness as well as an extinction and recovery, i.e. a reentrant behavior, of superconductivity. Especially, the latter is necessary to obtain a spin-valve with a large critical temperature shift between the parallel and antiparallel configurations of magnetizations in the F layers.
