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A determination of the superconducting (SC) electron pairing symmetry forms the basis for establishing a microscopic mechansim for superconductivity. For iron pnictide superconductors, the $s^pm$-pairing symmetry theory predicts the presence of a sha rp neutron spin resonance at an energy below the sum of hole and electron SC gap energies ($Eleq 2Delta$) below $T_c$. On the other hand, the $s^{++}$-pairing symmetry expects a broad spin excitation enhancement at an energy above $2Delta$ below $T_c$. Although the resonance has been observed in iron pnictide superconductors at an energy below $2Delta$ consistent with the $s^pm$-pairing symmetry, the mode has also be interpreted as arising from the $s^{++}$-pairing symmetry with $Ege 2Delta$ due to its broad energy width and the large uncertainty in determining the SC gaps. Here we use inelastic neutron scattering to reveal a sharp resonance at E=7 meV in SC NaFe$_{0.935}$Co$_{0.045}$As ($T_c = 18$ K). On warming towards $T_c$, the mode energy hardly softens while its energy width increases rapidly. By comparing with calculated spin-excitations spectra within the $s^{pm}$ and $s^{++}$-pairing symmetries, we conclude that the ground-state resonance in NaFe$_{0.935}$Co$_{0.045}$As is only consistent with the $s^{pm}$-pairing, and is inconsistent with the $s^{++}$-pairing symmetry.
The magnetic excitations in the paramagnetic-tetragonal phase of underdoped Ba(Fe0.953Co0.047)2As2, as measured by inelastic neutron scattering, can be well described by a phenomenological model with purely diffusive spin dynamics. At low energies, t he spectrum around the magnetic ordering vector Q_AFM consists of a single peak with elliptical shape in momentum space. At high energies, this inelastic peak is split into two peaks across the direction perpendicular to Q_AFM. We use our fittings to argue that such a splitting is not due to incommensurability or propagating spin-wave excitations, but is rather a consequence of the anisotropies in the Landau damping and in the magnetic correlation length, both of which are allowed by the tetragonal symmetry of the system. We also measure the magnetic spectrum deep inside the magnetically-ordered phase, and find that it is remarkably similar to the spectrum of the paramagnetic phase, revealing the strongly overdamped character of the magnetic excitations.
112 - Y. Xiao , Y. Su , H.-F. Li 2010
KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of KCrF3 compou nd are investigated by using polarized and unpolarized neutron powder diffraction methods. The results show that the KCrF3 compound crystallizes in tetragonal structure at room temperature and undergoes a monoclinic distortion with the decrease in temperature. The distortion of the crystal structure indicates the presence of cooperative Jahn-Teller distortion which is driven by orbital ordering. With decreasing temperature, four magnetic phase transitions are observed at 79.5, 45.8, 9.5, and 3.2 K, which suggests a rich magnetic phase diagram. Below T_N = 79.5 K, the Cr2+ moment orders in an incommensurate antiferromagnetic arrangement, which can be defined by the magnetic propagation vector (1/2$pm,$$delta,$, 1/2$pm,$$delta,$, 0). The incommensurate-commensurate magnetic transition occurs at 45.8 K and the magnetic propagation vector locks into (1/2, 1/2, 0) with the Cr moment of 3.34(5) $mu_B ,$ aligned ferromagnetically in (220) plane, but antiferromagnetically along [110] direction. Below 9.5 K, the canted antiferromagnetic ordering and weak ferromagnetism arise from the collinear antiferromagnetic structure, while the Dzyaloshinskii-Moriya interaction and tilted character of the single-ion anisotropy might give rise to the complex magnetic behaviors below 9.5 K.
75 - H.-F. Li , C. Broholm , D. Vaknin 2010
Inelastic neutron scattering from superconducting (SC) Ba(Fe$_{0.926}$Co$_{0.074}$)$_2$As$_2$ reveals anisotropic and quasi-two-dimensional (2D) magnetic excitations close to textbf{Q}$_{texttt{AFM}}=({1}{2}/{1}{2})$ - the 2D antiferromagnetic (AFM) wave-vector of the parent BaFe$_2$As$_2$ compound. The correlation length anisotropy of these low energy fluctuations is consistent with spin nematic correlations in the $J_1$-$J_2$ model with $J_1/J_2 sim$ 1. The spin resonance at $sim$8.3 meV in the SC state displays the same anisotropy. The anisotropic fluctuations experimentally evolve into two distinct maxima only along the direction transverse to textbf{Q}$_{texttt{AFM}}$ above $sim$80 meV indicating unusual quasi-propagating excitations.
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