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We have exposed a dual-phase Liquid Argon Time Projection Chamber (LAr-TPC) to a low energy pulsed narrowband neutron beam, produced at the Notre Dame Institute for Structure and Nuclear Astrophysics to study the scintillation light yield of recoilin g nuclei in a LAr-TPC. A liquid scintillation counter was arranged to detect and identify neutrons scattered in the LAr-TPC target and to select the energy of the recoiling nuclei. We report the observation of a significant dependence on drift field of liquid argon scintillation from nuclear recoils of 11 keV. This observation is important because, to date, estimates of the sensitivity of noble liquid TPC dark matter searches are based on the assumption that electric field has only a small effect on the light yield from nuclear recoils.
We report on the performance and commissioning of a cryogenic distillation column for low radioactivity underground argon at Fermi National Accelerator Laboratory. The distillation column is designed to accept a mixture of argon, helium, and nitrogen and return pure argon with a nitrogen contamination less than 10 ppm. In the first commissioning, we were able to run the distillation column in a continuous mode and produce argon that is 99.9% pure. After running in a batch mode, the argon purity was increased to 99.95%, with 500 ppm of nitrogen remaining. The efficiency of collecting the argon from the gas mixture was between 70% and 81%, at an argon production rate of 0.84-0.98 kg/day.
We report on the first large-scale production of low radioactivity argon from underground gas wells. Low radioactivity argon is of general interest, in particular for the construction of large scale WIMP dark matter searches and detectors of reactor neutrinos for non-proliferation efforts. Atmospheric argon has an activity of about 1 Bq/kg from the decays of 39Ar; the concentration of 39Ar in the underground argon we are collecting is at least a factor of 100 lower than this value. The argon is collected from a stream of gas from a CO2 well in southwestern Colorado with a Vacuum Pressure Swing Adsorption (VPSA) plant. The gas from the well contains argon at a concentration of 400-600 ppm, and the VPSA plant produces an output stream with an argon concentration at the level of 30,000-50,000 ppm (3-5%) in a single pass. This gas is sent for further processing to Fermilab where it is purified by cryogenic distillation. The argon production rate is presently 0.5 kg/day.
Neutrinoless double-beta decay experiments can potentially determine the Majorana or Dirac nature of the neutrino, and aid in understanding the neutrino absolute mass scale and hierarchy. Future 76Ge-based searches target a half-life sensitivity of > 10^27 y to explore the inverted neutrino mass hierarchy. Reaching this sensitivity will require a background rate of <1 count tonne^-1 y^-1 in a 4-keV-wide spectral region of interest surrounding the Q value of the decay. We investigate the overburden required to reach this background goal in a tonne-scale experiment with a compact (copper and lead) shield based on Monte Carlo calculations of cosmic-ray background rates. We find that, in light of the presently large uncertainties in these types of calculations, a site with an underground depth >~5200 mwe is required for a tonne-scale experiment with a compact shield similar to the planned 40-kg MAJORANA DEMONSTRATOR. The required overburden is highly dependent on the chosen shielding configuration and could be relaxed significantly if, for example, a liquid cryogen and water shield, or an active neutron shield were employed. Operation of the MAJORANA DEMONSTRATOR and GERDA detectors will serve to reduce the uncertainties on cosmic-ray background rates and will impact the choice of shielding style and location for a future tonne-scale experiment. 4/2013: The peer review process revealed that one of the veto rejection factors (the factor-of-4 described on p12) needs to be better established. Our reevaluation of this parameter to date has not yielded strong support for the value stated in the manuscript, and we require further study to develop a solid estimate. This further study will supersede the work described in this manuscript, and may or may not lead to the same conclusion regarding the ~>5200 mwe requirement for future tonne-scale 76Ge neutrinoless double beta decay experiments.
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