We have performed detailed $^{57}$Fe Mossbauer spectroscopy measurements on Ba$_{0.78}$K$_{0.22}$Fe$_2$As$_2$ and BaFe$_{2-x}$Ni$_x$As$_2$ single crystal mosaics showing antiferromagnetic ordering below $T_N$ with superconductivity below $T_C$. Analy
sis of the Mossbauer spectra shows a decrease in the magnetic hyperfine (hf) field but no change in the magnetic volume fraction below $T_C$. This clearly indicates the coexistence of magnetism and superconductivity in these compounds. The decrease in the magnetic hf field below $T_C$ depends on the difference between $T_N$ and $T_C$, being the largest for $T_N$ close to $T_C$. Two different explanations for this observation are given. We also find that the non-magnetic volume fraction below $T_N$ correlates with the Ni doping $x$, being large for high $T_C$ and small for high $T_N$.
We have studied the magnetism in superconducting single crystals of EuFe2 As1.4 P0.6 by using the local probe techniques of zero-field muon spin rotation/relaxation and 151 Eu/57 Fe Mossbauer spec- troscopy. All of these measurements reveal magnetic
hyperfine fields below the magnetic ordering temperature TM = 18 K of the Eu2+ moments. The analysis of the data shows that there is a coexistence of ferromagnetism, resulting from Eu2+ moments ordered along the crystallographic c-axis, and superconductivity below TSC approx 15 K. We find indications for a change in the dynamics of the small Fe magnetic moments (sim 0.07 mu B) at the onset of superconductivity: below TSC the Fe magnetic moments seem to be frozen within the ab-plane.
Pb films embedded with homogeneously distributed cobalt (Co) nanoparticles (mean size 4.5 nm) have been prepared. Previous transport investigations have shown that Co particles induce spontaneous vortices below the superconducting transition temperat
ure (T$_{c}$) in zero external magnetic field. In this paper we study in detail the influence of the Co volume franction and an external magnetic field on the superconducting transition in such composites. The large difference in T$_c$-reduction between the as-prepared and annealed samples can be attributed to the different superconducting coherence lengths and the resulting different diameters of the spontaneous vortices in these samples.
A hybrid system which consists of a superconducting (SC) Pb film (100 nm thickness) containing $sim$1 vol% single domain ferromagnetic (FM) Co particles of mean-size $sim$4.5 nm reveal unusual magnetic properties: (i) a controlled switching between t
he usual diamagnetic and the unusual paramagnetic Meissner effect in field cooling as well as in zero-field cooling experiments (ii) amplification of the positive magnetization when the sample enters the SC state below T$_c$. These experimental findings can be explained by the formation of spontaneous vortices and the possible alignment of these vortices due to the foregoing alignment of the Co particle FM moments by an external magnetic field.
The interplay between superconductivity and magnetism gives rise to many intriguing and exciting phenomena. In this Letter we report about a novel manifestation of this interplay: a temperature induced phase transition between different spontaneous v
ortex phases in lead superconducting films with embedded magnetic nanoparticles. Unlike common vortices in superconductors the vortex phase appears without any applied magnetic field. The vortices nucleate exclusively due to the stray field of the magnetic nanoparticles, which serve the dual role of providing the internal field and simultaneously acting as pinning centers. As in usual superconductors, one can move the spontaneous vortices with an applied electric current. Transport measurements reveal dynamical phase transitions that depend on temperature (T) and applied field (H) and support the obtained (H-T) phase diagram. In particular, we used a scaling analysis to characterize a transition from a liquid to a novel disordered solid resembling a vortex glass.
