We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice can be ma
pped to a spin-1 spatially anisotropic triangular lattice. The magnetization curve exhibits gapped behavior indicative of a dominant one-dimensional (1D) AF correlation. In the field-induced gapless phase, the specific heat and magnetic susceptibility show a phase transition to an ordered state with 2D characteristics. These results indicate that the spin-1 Haldane state is extended to the 2D system. We demonstrate that the gapped ground state observed in the present spin-1/2 frustrated square lattice originates from the one-dimensionalization caused by frustration.
We report the first (in)elastic scattering measurement of $^{25}mathrm{Al}+p$ with the capability to select and measure in a broad energy range the proton resonances in $^{26}$Si contributing to the $^{22}$Mg$(alpha,p)$ reaction at type I x-ray burst
energies. We measured spin-parities of four resonances above the $alpha$ threshold of $^{26}$Si that are found to strongly impact the $^{22}$Mg$(alpha,p)$ rate. The new rate advances a state-of-the-art model to remarkably reproduce lightcurves of the GS 1826$-$24 clocked burster with mean deviation $<$9 % and permits us to discover a strong correlation between the He abundance in the accreting envelope of photospheric radius expansion burster and the dominance of $^{22}$Mg$(alpha,p)$ branch.
We present a model compound with a spin-1/2 spatially anisotropic frustrated square lattice, in which three antiferromagnetic interactions and one ferromagnetic interaction are competing. We observe an unconventional gradual increase in the low-tempe
rature magnetization curve reminiscent of the quantum critical behavior between gapped and gapless phases. In addition, the specific heat and electron spin resonance signals indicate one-dimensional characteristics. These results demonstrate quantum critical behavior associated with one dimensionalization caused by frustrated interactions in the spin-1/2 spatially anisotropic square lattice.
We present a mixed spin-(1/2, 5/2) chain composed of a charge-transfer salt (4-Br-$o$-MePy-V)FeCl$_4$. We observe the entire magnetization curve up to saturation, which exhibits a clear Lieb-Mattis magnetization plateau and subsequent quantum phase t
ransition towards the gapless Luttinger-liquid phase. The observed magnetic behavior is quantitatively explained by a mixed spin-(1/2, 5/2) chain model. The present results demonstrate a quantum many-body effect based on quantum topology and provide a new stage in the search for topological properties in condensed matter physics.
We present a new model compound with the S = 1/2 frustrated square lattice composed of the charge-transfer salt (o-MePy-V)PF6. Ab initio calculations indicate the formation of an S = 1/2 square lattice, in which six types of nearest-neighbor ferromag
netic- and antiferromagnetic interactions cause frustration. By applying a magnetic field, we observe an unusually gradual increase of magnetization and a subsequent 1/2-plateau-like behavior. A numerical analysis using the tensor network method qualitatively demonstrates such behaviors and suggests a collinear ordered state and a field-enhanced quantum fluctuation. Furthermore, the local magnetization and T1^-1 probed by nuclear magnetic resonance measurements support these findings.
High-resolution spectroscopy of the core of the Perseus Cluster of galaxies, using the $Hitomi$ satellite above 2 keV and the $XMM$-$Newton$ Reflection Grating Spectrometer at lower energies, provides reliable constraints on the abundances of O, Ne,
Mg, Si, S, Ar, Ca, Cr, Mn, Fe, and Ni. Accounting for all known systematic uncertainties, the Ar/Fe, Ca/Fe, and Ni/Fe ratios are determined with a remarkable precision of less than 10%, while the constraints on Si/Fe, S/Fe, and Cr/Fe are at the 15% level, and Mn/Fe is measured with a 20% uncertainty. The average biases in determining the chemical composition using archival CCD spectra from $XMM$-$Newton$ and $Suzaku$ range typically from 15-40%. A simple model in which the enrichment pattern in the Perseus Cluster core and the proto-solar nebula are identical gives a surprisingly good description of the high-resolution X-ray spectroscopy results, with $chi^2=10.7$ for 10 d.o.f. However, this pattern is challenging to reproduce with linear combinations of existing supernova nucleosynthesis calculations, particularly given the precise measurements of intermediate $alpha$-elements enabled by $Hitomi$. We discuss in detail the degeneracies between various supernova progenitor models and explosion mechanisms, and the remaining uncertainties in these theoretical models. We suggest that including neutrino physics in the core-collapse supernova yield calculations may improve the agreement with the observed pattern of $alpha$-elements in the Perseus Cluster core. Our results provide a complementary benchmark for testing future nucleosynthesis calculations required to understand the origin of chemical elements.
We present a quantu spin liquid state in a spin-1/2 honeycomb lattice with randomness in the exchange interaction. That is, we successfully introduce randomness into the organic radial-based complex and realize a random-singlet (RS) state. All magnet
ic and thermodynamic experimental results indicate the liquid-like behaviors, which are consistent with those expected in the RS state. These results demonstrate that the randomness or inhomogeneity in the actual systems stabilize the RS state and yield liquid-like behavior.
Background: Type I x-ray bursts are the most frequent thermonuclear explosions in the galaxy, resulting from thermonuclear runaway on the surface of an accreting neutron star. The $^{30}$S($alpha$,p) reaction plays a critical role in burst models, ye
t insufficient experimental information is available to calculate a reliable, precise rate for this reaction. Purpose: Our measurement was conducted to search for states in $^{34}$Ar and determine their quantum properties. In particular, natural-parity states with large $alpha$-decay partial widths should dominate the stellar reaction rate. Method: We performed the first measurement of $^{30}$S+$alpha$ resonant elastic scattering up to a center-of-mass energy of 5.5 MeV using a radioactive ion beam. The experiment utilized a thick gaseous active target system and silicon detector array in inverse kinematics. Results: We obtained an excitation function for $^{30}$S($alpha$,$alpha$) near $150^{circ}$ in the center-of-mass frame. The experimental data were analyzed with an $R$-Matrix calculation, and we observed three new resonant patterns between 11.1 and 12.1 MeV, extracting their properties of resonance energy, widths, spin, and parity. Conclusions: We calculated the resonant thermonuclear reaction rate of $^{30}$S($alpha$,p) based on all available experimental data of $^{34}$Ar and found an upper limit about one order of magnitude larger than a rate determined using a statistical model. The astrophysical impact of these two rates has been investigated through one-zone postprocessing type I x-ray burst calculations. We find that our new upper limit for the $^{30}$S($alpha$,p)$^{33}$Cl rate significantly affects the predicted nuclear energy generation rate during the burst.
It is a well-known fact that a cluster of nucleons can be formed in the interior of an atomic nucleus, and such clusters may occupy molecular-like orbitals, showing characteristics similar to normal molecules consisting of atoms. Chemical molecules h
aving a linear alignment are commonly seen in nature, such as carbon dioxide. A similar linear alignment of the nuclear clusters, referred to as linear-chain cluster state (LCCS), has been studied since the 1950s, however, up to now there is no clear experimental evidence demonstrating the existence of such a state. Recently, it was proposed that an excess of neutrons may offer just such a stabilizing mechanism, revitalizing interest in the nuclear LCCS, specifically with predictions for their emergence in neutron-rich carbon isotopes. Here we present the experimental observation of {alpha}-cluster states in the radioactive 14C nucleus. Using the 10Be+{alpha} resonant scattering method with a radioactive beam, we observed a series of levels which completely agree with theoretically predicted levels having an explicit linear-chain cluster configuration. We regard this as the first strong indication of the linear-chain clustered nucleus.
We present the first experimental realization of an $S=2$ ferromagnetic-antiferromagnetic (F-AF) alternating chain in a new Mn-verdazyl complex [Mn(hfac)$_2$]$cdot$($o$-Py-V) [hfac=1,1,1,5,5,5-hexafluoroacetylacetonate; $o$-Py-V=3-(2-pyridyl)-1,5-dip
henylverdazyl]. Through the $ab$ $initio$ molecular orbital calculation, magnetization, and ESR measurements, this compound is confirmed to form an $S=2$ F-AF alternating chain with Ising anisotropy below about 100 K. Furthermore, we find an anomalous change in magnetization at 1/4 of the saturation value, which is probably a manifestation of the quantum nature of the system.
