Magneto-optical transitions between Landau levels can provide precise spectroscopic information on the electronic structure and excitation spectra of graphene, enabling probes of substrate and many-body effects. We calculate the magneto-optical condu
ctivity of large-size graphene flakes using a tight-binding approach. Our method allows us to directly compare the magneto-optical response of an isolated graphene flake with one aligned on hexagonal boron nitride giving rise to a periodic superlattice potential. The substrate interaction induces band gaps away from the Dirac point. In the presence of a perpendicular magnetic field Landau-level like structures emerge from these zero-field band gaps. The energy dependence of these satellite structures is, however, not easily accessible by conventional probes of the density of states by varying the back-gate voltage. Here we propose the magneto-optical probing of the superlattice perturbed spectrum. Our simulation includes magneto-excitonic effects in first-order perturbation theory. Our approach yields a quantitative explanation of recently observed Landau-level dependent renormalizations of the Fermi velocity.
Graphene flakes placed on hexagonal boron nitride feature in the presence of a magnetic field a complex electronic structure due to a hexagonal moire potential resulting from the van der Waals interaction with the substrate. The slight lattice mismat
ch gives rise to a periodic supercell potential. Zone folding is expected to create replica of the original Dirac cone and Hofstadter butterflies. Our large-scale tight binding simulation reveals an unexpected coexistence of a relativistic and non-relativistic Landau level structure. The presence of the zeroth Landau level and its associated butterfly is shown to be the unambiguous signature for the occurrence of Dirac cone replica.
Using low-temperature scanning tunneling spectroscopy, we map the local density of states (LDOS) of graphene quantum dots supported on Ir(111). Due to a band gap in the projected Ir band structure around the graphene K point, the electronic propertie
s of the QDs are dominantly graphene-like. Indeed, we compare the results favorably with tight binding calculations on the honeycomb lattice based on parameters derived from density functional theory. We find that the interaction with the substrate near the edge of the island gradually opens a gap in the Dirac cone, which implies soft-wall confinement. Interestingly, this confinement results in highly symmetric wave functions. Further influences of the substrate are given by the known moir{e} potential and a 10% penetration of an Ir surface resonance
We investigate the addition spectrum of a graphene quantum dot in the vicinity of the electron-hole crossover as a function of perpendicular magnetic field. Coulomb blockade resonances of the 50 nm wide dot are visible at all gate voltages across the
transport gap ranging from hole to electron transport. The magnetic field dependence of more than 50 states displays the unique complex evolution of the diamagnetic spectrum of a graphene dot from the low-field regime to the Landau regime with the n=0 Landau level situated in the center of the transport gap marking the electron-hole crossover. The average peak spacing in the energy region around the crossover decreases with increasing magnetic field. In the vicinity of the charge neutrality point we observe a well resolved and rich excited state spectrum.
We present realistic simulations of quantum confinement effects in ballistic graphene quantum dots with linear dimensions of 10 to 40 nm. We determine wavefunctions and energy level statistics in the presence of disorder resulting from edge roughness
, charge impurities, or short-ranged scatterers. Marked deviations from a simple Dirac billiard for massless fermions are found. We find a remarkably stable dependence of the nearest-neighbor level spacing on edge roughness suggesting that the roughness of fabricated devices can be potentially characterized by the distribution of measured Coulomb blockade peaks.
