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129 - R. Wallauer , S. Sanna , E. Lahoud 2015
Angle-resolved photoemission spectroscopy (ARPES) is one of most powerful techniques to unravel the electronic properties of layered materials and in the last decades it has lead to a significant progress in the understanding of the band structures o f cuprates, pnictides and other materials of current interest. On the other hand, its application to Mott-Hubbard insulating materials where a Fermi surface is absent has been more limited. Here we show that in these latter materials, where electron spins are localized, ARPES may provide significant information on the spin correlations which can be complementary to the one derived from neutron scattering experiments. Sr$_2$Cu$_{1-x}$Zn$_x$O$_2$Cl$_2$, a prototype of diluted spin $S=1/2$ antiferromagnet (AF) on a square lattice, was chosen as a test case and a direct correspondence between the amplitude of the spectral weight beyond the AF zone boundary derived from ARPES and the spin correlation length $xi$ estimated from $^{35}$Cl NMR established. It was found even for correlation lengths of a few lattice constants a significant spectral weight in the back-bended band is present which depends markedly on $xi$. Moreover the temperature dependence of that spectral weight is found to scale with the $x$ dependent spin-stiffness. These findings prove that ARPES technique is very sensitive to short-range correlations and its relevance in the understanding of the electronic correlations in cuprates is discussed.
We measured the electronic structure of Fe substituted Bi2212 using Angle Resolved Photoemission Spectroscopy (ARPES). We find that the substitution does not change the momentum dependence of the superconducting gap but induces a very anisotropic enh ancement of the scattering rate. A comparison of the effect of Fe substitution to that of Zn substitution suggests that the Fe reduces T$_c$ so effectively because it supresses very strongly the coherence weight around the anti-nodes.
In an ideal bulk topological-insulator (TI) conducting surface states protected by time reversal symmetry enfold an insulating crystal. However, the archetypical TI, Bi2Se3, is actually never insulating; it is in fact a relatively good metal. Neverth eless, it is the most studied system among all the TIs, mainly due to its simple band-structure and large spin-orbit gap. Recently it was shown that copper intercalated Bi2Se3 becomes superconducting and it was suggested as a realization of a topological superconductor (TSC). Here we use a combination of techniques that are sensitive to the shape of the Fermi surface (FS): the Shubnikov-de Haas (SdH) effect and angle resolved photoemission spectroscopy (ARPES) to study the evolution of the FS shape with carrier concentration, n. We find that as n increases, the FS becomes 2D-like. These results are of crucial importance for understanding the superconducting properties of CuxBi2Se3.
We report point contact measurements in high quality single crystals of Cu0.2Bi2Se3. We observe three different kinds of spectra: (1) Andreev-reflection spectra, from which we infer a superconducting gap size of 0.6mV; (2) spectra with a large gap wh ich closes above Tc at about 10K; and (3) tunneling-like spectra with zero-bias conductance peaks. These tunneling spectra show a very large gap of ~2meV (2Delta/KTc ~ 14).
Point contact conductance measurements on topological $Bi_2Te_2Se$ and $Bi_2Se_3$ films reveal a signature of superconductivity below 2-3 K. In particular, critical current dips and a robust zero bias conductance peak are observed. The latter suggest s the presence of zero energy bound states which could be assigned to Majorana Fermions in an unconventional topological superconductor. We attribute these novel observations to proximity induced local superconductivity in the films by small amounts of superconducting Bi inclusions or segregation to the surface, and provide supportive evidence for these effects.
We measured the electronic-structure of FeSe_xTe_1-x above and below Tc. In the normal state we find multiple bands with remarkably small values for the Fermi energy, E_F. Yet,below Tc we find a superconducting gap, Delta, that is comparable in size to E_F, leading to a ratio Delta/E_F~0.5 that is much larger than found in any previously studied superconductor. We also observe an anomalous dispersion of the coherence peak which is very similar to the dispersion found in cold Fermi-gas experiments and which is consistent with the predictions of the BCS-BEC crossover theory.
Shubnikov-de Haas (SdH) oscillations are observed in Bi2Se3 flakes with high carrier concentration and low bulk mobility. These oscillations probe the protected surface states and enable us to extract their carrier concentration, effective mass and D ingle temperature. The Fermi momentum obtained is in agreement with angle resolved photoemission spectroscopy (ARPES) measurements performed on crystals from the same batch. We study the behavior of the Berry phase as a function of magnetic field. The standard theoretical considerations fail to explain the observed behavior.
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