Third-harmonic generation (THG) experiments on superconductors can be used to investigate collective excitations like the amplitude mode of the order parameter known as Higgs mode. These modes are visible due to resonances in the THG signal if the dr
iving frequency matches the energy of the mode. In real materials multiple modes can exist giving rise to additional THG contributions, such that it is difficult to unambiguously interpret the results. In this paper, we additionally analyze the phase of the THG signal, which contains microscopic details beyond classical resonances as well as signatures of couplings between modes which are difficult to observe in the amplitude alone. We investigate how the Higgs mode, impurities or Coulomb interaction affects the phase response and consider exemplary two systems with additional modes. We argue that extracting this phase information could be valuable in future experiments.
Recent studies have emphasized the importance of impurity scattering for the optical Higgs response of superconductors. In the dirty limit, an additional paramagnetic coupling of light to the superconducting condensate arises which drastically enhanc
es excitation. So far, most work concentrated on the periodic driving with light, where the third-harmonic generation response of the Higgs mode was shown to be enhanced. In this work, we additionally calculate the time-resolved optical conductivity of single- and two-band superconductors in a two-pulse quench-probe setup, where we find good agreement with existing experimental results. We use the Mattis-Bardeen approach to incorporate impurity scattering and calculate explicitly the time-evolution of the system. Calculations are performed both in a diagrammatic picture derived from an effective action formalism and within a time-dependent density matrix formalism.
The anomalous proximity effect in dirty superconducting junctions is one of most striking phenomena highlighting the profound nature of Majorana bound states and odd-frequency Cooper pairs in topological superconductors. Motivated by the recent exper
imental realization of planar topological Josephson junctions, we describe the anomalous proximity effect in a superconductor/semiconductor hybrid, where an additional dirty normal-metal segment is extended from a topological Josephson junction. The topological phase transition in the topological Josephson junction is accompanied by a drastic change in the low-energy transport properties of the attached dirty normal-metal. The quantization of the zero-bias differential conductance, which appears only in the topologically nontrivial phase, is caused by the penetration of the Majorana bound states and odd-frequency Cooper pairs into a dirty normal-metal segment. As a consequence, we propose a practical experiment for observing the anomalous proximity effect.
Josephson junctions based on three-dimensional topological insulators offer intriguing possibilities to realize unconventional $p$-wave pairing and Majorana modes. Here, we provide a detailed study of the effect of a uniform magnetization in the norm
al region: We show how the interplay between the spin-momentum locking of the topological insulator and an in-plane magnetization parallel to the direction of phase bias leads to an asymmetry of the Andreev spectrum with respect to transverse momenta. If sufficiently large, this asymmetry induces a transition from a regime of gapless, counterpropagating Majorana modes to a regime with unprotected modes that are unidirectional at small transverse momenta. Intriguingly, the magnetization-induced asymmetry of the Andreev spectrum also gives rise to a Josephson Hall effect, that is, the appearance of a transverse Josephson current. The amplitude and current phase relation of the Josephson Hall current are studied in detail. In particular, we show how magnetic control and gating of the normal region can enable sizable Josephson Hall currents compared to the longitudinal Josephson current. Finally, we also propose in-plane magnetic fields as an alternative to the magnetization in the normal region and discuss how the planar Josephson Hall effect could be observed in experiments.
Higgs oscillations in nonequilibrium superconductors provide an unique tool to obtain information about the underlying order parameter. Several properties like the absolute value, existence of multiple gaps and the symmetry of the order parameter can
be encoded in the Higgs oscillation spectrum. Studying Higgs oscillations with time-resolved angle-resolved photoemission spectroscopy (ARPES) has the advantage over optical measurements that a momentum-resolved analysis of the condensate dynamic is possible. In this paper, we investigate the time-resolved spectral function measured in ARPES for different quench protocols. We find that analyzing amplitude oscillations of the ARPES intensity in the whole Brillouin zone allows to understand how the condensate dynamic contributes to the emerging of collective Higgs oscillations. Furthermore, by evaluating the phase of these oscillations the symmetry deformation dynamic of the condensate can be revealed, which gives insight about the ground state symmetry of the system. With such an analysis, time-resolved ARPES experiments might be used in future as a powerful tool in the field of Higgs spectroscopy.
Higgs spectroscopy is a new field in which Higgs modes in nonequilibrium superconductors are analyzed to gain information about the ground state. One experimental setup in which the Higgs mode in s-wave superconductors was observed is periodic drivin
g with THz light, which shows resonances in the third-harmonic generation (THG) signal if twice the driving frequency matches the energy of the Higgs mode. We derive expressions of the driven gap oscillations for arbitrary gap symmetry and calculate the THG response. We demonstrate that the possible Higgs modes for superconductors with non-trivial gap symmetry can lead to additional resonances if twice the driving frequency matches the energy of these Higgs modes and we disentangle the influence of charge density fluctuations (CDF) to the THG signal within our clean-limit analysis. With this we show that THG experiments on unconventional superconductors allow for a detection of their Higgs modes. This paves the way for future studies on realistic systems including additional features to understand the collective excitation spectra of unconventional superconductors.
When charge current passes through a normal metal that exhibits spin Hall effect, spin accumulates at the edge of the sample in the transverse direction. We predict that this spin accumulation, or spin voltage, enables quantum tunneling of spin throu
gh an insulator or vacuum to reach a ferromagnet without transferring charge. In a normal metal/insulator/ferromagnetic insulator trilayer (such as Pt/oxide/YIG), the quantum tunneling explains the spin-transfer torque and spin pumping that exponentially decay with the thickness of the insulator. In a normal metal/insulator/ferromagnetic metal trilayer (such as Pt/oxide/Co), the spin transfer in general does not decay monotonically with the thickness of the insulator. Combining with the spin Hall magnetoresistance, this tunneling mechanism points to the possibility of a new type of tunneling spectroscopy that can probe the magnon density of states of a ferromagnetic insulator in an all-electrical and noninvasive manner.
We formulate a kinetic theory for non-centrosymmetric superconductors at low temperatures in the clean limit. The transport equations are solved quite generally in spin- and particle-hole (Nambu) space by performing first a transformation into the ba
nd basis and second a Bogoliubov transformation to the quasiparticle-quasihole phase space. Our result is a particle-hole-symmetric, gauge-invariant and charge conserving description, which is valid in the whole quasiclassical regime. We calculate the current response, the specific heat capacity, and the Raman response function. For the Raman case, we investigate within this framework the polarization-dependence of the electronic (pair-breaking) Raman response for the recently discovered non-centrosymmetric superconductors at zero temperature. Possible applications include the systems CePt$_3$Si and Li$_2$Pd$_x$Pt$_{3-x}$B, which reflect the two important classes of the involved spin-orbit coupling. We provide analytical expressions for the Raman vertices for these two classes and calculate the polarization-dependence of the electronic spectra. We predict a two-peak structure and different power laws with respect to the unknown relative magnitude of the singlet and triplet contributions to the superconducting order parameter, revealing a large variety of characteristic fingerprints of the underlying condensate.
We formulate a theory for the polarization-dependence of the electronic (pair-breaking) Raman response for the recently discovered non-centrosymmetric superconductors in the clean limit at zero temperature. Possible applications include the systems C
ePt$_3$Si and Li$_2$Pd$_x$Pt$_{3-x}$B which reflect the two important classes of the involved spin-orbit coupling. We provide analytical expressions for the Raman vertices for these two classes and calculate the polarization dependence of the electronic spectra. We predict a two-peak structure and different power laws with respect to the unknown relative magnitude of the singlet and triplet contributions to the superconducting order parameter, revealing a large variety of characteristic fingerprints of the underlying condensate.
Using a generalized response theory we derive the electronic Raman response function for metals with anisotropic relaxation rates. The calculations account for the long--range Coulomb interaction and treat the collision operator within a charge conse
rving relaxation time approximation. We extend earlier treatments to finite wavenumbers ($|{bf q}|ll k_{rm F}$) and incorporate inelastic electron--electron scattering besides elastic impurity scattering. Moreover we generalize the Lindhard density response function to the Raman case. Numerical results for the quasiparticle scattering rate and the Raman response function for cuprate superconductors are presented.
